Download or read book Photoelectron Distributions from Resonant Multiphoton Ionization of Atoms and Molecules written by James Stevenson Keller and published by . This book was released on 1989 with total page 460 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Multiphoton lonization of Atoms written by S.L. Chin and published by Elsevier. This book was released on 2012-12-02 with total page 287 pages. Available in PDF, EPUB and Kindle. Book excerpt: Multiphoton lonization of Atoms provides a pedagogical review of the whole subfield of multiphoton ionization of atoms. This book discusses the “normal multiphoton ionization of atoms; calculation of resonant multiphoton processes; and angular distribution of photoelectrons and light polarization effects in multiphoton ionization of atoms. The multiphoton ionization involving continuum-continuum transitions; creation of doubly charged strontium ions; and many-electron processes in nonlinear ionization of atoms are also elaborated. Other topics include the non-resonant multiphoton ionization of atoms; above-threshold ionization theory; autoionizing states in multiphoton transitions; and specific features of the spectra of alkaline-earth atoms. This publication is beneficial to physics students and researchers conducting work on the multiple ionization of atoms.
Download or read book High Resolution Spectroscopy and Dynamics of Multiphoton Processes in Atoms and Molecules written by P. M. Dehmer and published by . This book was released on 1984 with total page 16 pages. Available in PDF, EPUB and Kindle. Book excerpt: This report summarizes research on resonantly enhanced multiphoton absorption dissociation, and ionization processes in atoms and molecules. Multiphoton processes are studied using from one to three independently tunable visible and/or UV laser beams in order to establish both the underlying physics and the high degree of selectivity of multiphoton processes. Measurements are made to probe both the formation of excited molecular states and the subsequent behavior of excited states either in the presence or in the abscence of further intense laser radiation. Detection methods include laser-induced fluorescence, ion mass analysis, and electron energy analysis. During the current reporting period, we have studied resonant multiphoton ionization processes for the molecules N2, CO, O2, NO, NeXe, ArXe, KrXe, and Xe2 and for the atoms C, I, and S using both mass spectrometry and photoelectron spectroscopy to analyze the products of the ionizations. In addition, we are developing three new instruments that will provide significantly enhanced resolution, collection efficiency, and versatility in both the ion mass and the electron kinetic energy detection channels. Keywords include: double resonance spectroscopy, electron spectroscopy, molecular beams, rydberg states; photoelectron angular, distributions. (Author).
Download or read book Multiphoton Processes written by P. Lambropoulos and published by Springer Science & Business Media. This book was released on 2012-12-06 with total page 206 pages. Available in PDF, EPUB and Kindle. Book excerpt: The chapters of this volume represent the invited papers delivered at the 3rd International Conference on Multiphoton Processes (ICOMP III) held in Iraklion, Crete, Greece, September 5-11, 1984. The invited papers at a conference like ICOMP cannot possibly cover the whole field which has grown to immense proportions in recent years, overlapping with such diverse areas as atomic and molecular spectroscopy, plasma physics, nonlinear optics, quantum optics, etc. We believe these contributions represent that part of the research activity which has been attracting the most interest in the past year or so, as well as reviews of some of the more established topics. Even within this scope, and given the confines imposed by the fi nite duration of a conference, important and timely topics are inevitably left out. But then, there will be ICOMP IV. The collection of articles in this volume, combined with extensive ref erences to related work given by the authors, should provide an introduc tion to the major problems of the field and its state of the art. The chapters have been arranged according to thematic proximity, beginning with atoms, and continuing on with molecules and surfaces. This classi fication, however, would not cover all the subject matter even within the limited scope of the conference and of this volume.
Download or read book Resonant Multiphoton Ionization Spectra of Molecules and Molecular Fragments Annual Technical Report October 1987 September 1988 written by and published by . This book was released on 1988 with total page 13 pages. Available in PDF, EPUB and Kindle. Book excerpt: The objective of the research under this contract is to carry out studies of resonant enhanced multiphoton ionization (REMPI) processes in molecules. In the (n+1)-REMPI process of interest an atom or molecule in a specific initial state absorbs n photons making a transition to an intermediate state from which it is subsequently ionized by absorption of an additional photon. The studies are designed to provide a quantitatively robust analysis and prediction of key spectral features in several ongoing experimental studies and potentially practical applications of this technique. The specific problems of interest to the authors in these studied are (1) the vibrational distributions of ions that can be expected in REMPI of small molecules and molecular fragments with particular emphasis on their non-Franck-Condon behavior. Such non-Franck-Condon behavior introduces serious complications in the use of the technique for state-specific production of ions, e.g., O2([nu]) and OH([nu]), and in the extraction of state populations from REMPI signals, (2) rotational distributions of ions that can be produced in various REMPI schemes and how these distributions can be tuned by choice of the resonant state and influenced by the molecular character of the photoelectron, and (3) the circular dichroism in photoelectron angular distributions, i.e., the difference in photoelectron angular distributions produced by right- and left-circularly polarized, and their use as a probe of molecular alignment. Here the author will summarize the progress that has been made to date in the studies of these features and applications of REMPI of molecules and molecular fragments. A significant feature of these studies, which will be explicitly assumed throughout the discussion below, is that they are carried out using quantitatively reliable molecular photoelectron orbitals.
Download or read book Angular Distributions of Photoelectrons from Resonant Multiphoton Ionization written by Ring-Ling Chien and published by . This book was released on 1983 with total page 254 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Calculations of High Intensity Multiphoton Ionization and Photoemission from Atoms written by K. C. Kulander and published by . This book was released on 1992 with total page 4 pages. Available in PDF, EPUB and Kindle. Book excerpt: A method which involves the direct solution of the time dependent Schrodinger equations has been used in studies of the dynamics of excitation of and emission from atoms in intense, pulsed laser fields. A surprising array of effects have been observed during high-intensity, short-pulse laser excitation of atoms and molecules. To model the results of these measurements, we have developed methods to solve the time-dependent Schrodinger equation for an atom in a time varying, classical electromagnetic field. Studies on may atomic and molecular systems have been performed over a range of intensities from the regime within which perturbative techniques are valid up to field strengths well above an atomic unit (I> (3.51 x 10 to the 16th W)/sq. cm.). These calculations have provided predictions for ionization rates, 1 photoelectron energy and angular distributions and photoemission rates. The effects of ac Stark shifted and intensity broadened intermediate states on the emission processes have been investigated.
Download or read book Advances In Multi photon Processes And Spectroscopy Vol 4 written by Sheng-hsien Lin and published by World Scientific. This book was released on 1988-05-01 with total page 326 pages. Available in PDF, EPUB and Kindle. Book excerpt: Contents:Two-Color Double Resonance Spectroscopy For the Study of High Excited States of Molecules (M Ito & M Fujii)Resonantly Enhanced Multiphoton Ionization — Photoelectron Spectroscopy as a Probe of Molecular Photophysics and Photochemistry (S Pratt, P Dehmer & J Dehmer)Progress in Resonance Enhanced Multiphoton Ionization Spectroscopy of Transient Free Radicals (J Hudgens)Time-Resolved Resonance Raman Spectroscopy: Intense Electromagnetic Field Effects, and Photoelectrochemical Reactions on Semiconductor Crystallite Surfaces (L Brus) Readership: Atomic physicists, chemists and materials scientists.
Download or read book Photoelectron Angular Distributions for Cesium Rubidium and Sodium Atoms Using Multiphoton Ionization written by Adila Dodhy and published by . This book was released on 1985 with total page 214 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Photoelectron Angular Distributions from Two photon Ionizations of Atoms written by Louis Hamilton Haber and published by . This book was released on 2009 with total page 322 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Quantum Metrology with Photoelectrons written by Paul Hockett and published by Morgan & Claypool Publishers. This book was released on 2018-04-20 with total page 126 pages. Available in PDF, EPUB and Kindle. Book excerpt: Since the turn of the century, the increasing availability of photoelectron imaging experiments, along with the increasing sophistication of experimental techniques, and the availability of computational resources for analysis and numerics, has allowed for significant developments in such photoelectron metrology. Quantum Metrology with Photoelectrons, Volume 2: Applications and Advances discusses the fundamental concepts along with recent and emerging applications. Volume 2 explores the applications and development of quantum metrology schemes based on photoelectron measurements. The author begins with a brief historical background on "complete" photoionization experiments, followed by the details of state reconstruction methodologies from experimental measurements. Three specific applications of quantum metrology schemes are discussed in detail. In addition, the book provides advances, future directions, and an outlook including (ongoing) work to generalise these schemes and extend them to dynamical many-body systems. Volume 2 will be of interest to readers wishing to see the (sometimes messy) details of state reconstruction from photoelectron measurements as well as explore the future prospects for this class of metrology.
Download or read book Photoelectron angular distributions from fixed in space molecules written by Sofie Louise Kragh and published by . This book was released on 2010 with total page 85 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Resonant Multiphoton Ionization Spectra of Molecules and Molecular Fragments Technical Progress Report written by and published by . This book was released on 1997 with total page 8 pages. Available in PDF, EPUB and Kindle. Book excerpt: Objectives of this research are the development and application of theoretical techniques for studying several resonant multiphoton ionization processes in molecules. Specific problems of interest pertain to experimental studies of such spectra in which the photoelectron energy and angular distributions are determined.
Download or read book Coherence Phenomena in Atoms and Molecules in Laser Fields written by Andre D Bandrauk and published by Springer Science & Business Media. This book was released on 2012-12-06 with total page 397 pages. Available in PDF, EPUB and Kindle. Book excerpt: This volume contains the lectures and communications presented at the NATO Advanced Research Workshop (NATO ARW 900857) which was held May 5-10, 1991 at McMaster University, Hamilton, Ontario, Canada. A scientific commitee made up of P.P. Lambropoulos (USC & Crete), P.8. Corkum (NRC, Ottawa), and H. B. vL. van den Heuvell (FOM, Amsterdam) guided the organizers, A.D. Bandrauk (Sherbrooke) and S.C. Wallace (Toronto) in preparing a programme which would cover the latest advances in the field of atom and molecule laser interactions. Since the last meeting held in July 1987 on "Atomic and Molecular Processes with Short Intense Laser Pulses", NATO ASI vol 1718 (Plenum Press 1988), considerable progress has been made in understanding high intensity effects on atoms and the concomitant coherence effects. After four years, the emphasis is now shifting more to molecules. The present volume represents therefore this trend with four sections covering the main interests of research endeavours in this area: i) Atoms in Intense Laser-Fields ii) Molecules in Intense Laser Fields iii) Atomic Coherences iv) Molecular Coherences The experience developed over the years in multiphoton atomic processes has been very useful and is the main source of our understanding of similar processes in molecules. Thus ATI (above threshold ionization) has been found to occur in molecules as well as a new phenomenon, ATD (above-threshold dissociation). Laser-induced avoided crossings of molecular electronic surfaces is also now entering the current language of high intensity molecular processes.
Download or read book Molecular Multiphoton Ionization written by G. n GIBSON and published by . This book was released on 1992 with total page 7 pages. Available in PDF, EPUB and Kindle. Book excerpt: Resonant multiphoton ionization (MPI) of nitrogen has been studied using photoelectron spectroscopy in the short-pulse regime. Both Rydberg and valence states are identified as intermediate resonances in the photoionization process, although the valence states are seen only at low intensity. It is shown that the vibrational structure of the Rydberg states acting as intermediate resonances cancels out in the photoelectron spectrum, leading to sharp atomic-like spectra, even at high intensities. Finally, the ionization of the 3 sigma sub g 1 pi sub u and 2 sigma sub u electrons are clearly distinguished.
Download or read book Advances in Atomic and Molecular Physics written by and published by Academic Press. This book was released on 1988-08-01 with total page 341 pages. Available in PDF, EPUB and Kindle. Book excerpt: Advances in Atomic and Molecular Physics
Download or read book Photoionization and Photo Induced Processes in Mass Spectrometry written by Ralf Zimmermann and published by John Wiley & Sons. This book was released on 2021-07-06 with total page 448 pages. Available in PDF, EPUB and Kindle. Book excerpt: Provides comprehensive coverage of laser-induced ionization processes for mass spectrometry analysis Drawing on the expertise of the leading academic and industrial research groups involved in the development of photoionization methods for mass spectrometry, this reference for analytical scientists covers both the theory and current applications of photo-induced ionization processes. It places widely used techniques such as MALDI side by side with more specialist approaches such as REMPI and RIMS, and discusses leading edge developments in ultrashort laser pulse desorption, to give readers a complete picture of the state of the technology. Photoionization and Photo-Induced Processes in Mass Spectrometry: Fundamentals and Applications starts with a complete overview of the fundamentals of the technique, covering the basics of the gas phase ionization as well as those of laser desorption and ablation, pulse photoionization, and single particle ionization. Numerous application examples from different analytical fields are described that showcase the power and the wide scope of photo ionization in mass spectrometry. -The first general reference book on photoionization techniques for mass spectrometry -Examines technologies and applications of gas phase resonance-enhanced multiphoton ionization mass spectrometry (REMPI-MS) and gas phase resonance ionization mass spectrometry (RIMS) -Provides complete coverage of popular techniques like MALDI -Discusses the current and potential applications of each technology, focusing on process and environmental analysis Photoionization and Photo-Induced Processes in Mass Spectrometry: Fundamentals and Applications is an excellent book for spectroscopists, analytical chemists, photochemists, physical chemists, and laser specialists.
