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Book Evaluation of In plant Neutron Coincidence Counters for the Measurement of Molten Salt Extraction Residues

Download or read book Evaluation of In plant Neutron Coincidence Counters for the Measurement of Molten Salt Extraction Residues written by and published by . This book was released on 1993 with total page 8 pages. Available in PDF, EPUB and Kindle. Book excerpt: Americium is extracted from plutonium by a molten salt extraction (MSE) process. The residual americium-laden salts are a significant waste stream in this pyrochemical purification process. Rapid assay of MSE residues is desirable to minimize the exposure of personnel to these often high-level emissions. However, the quantitative assay of plutonium in MSE residues is difficult. Variable, unknown (a, n) rates and variable emitted-neutron energy spectra preclude the use of standard neutron coincidence counting techniques with old-generation neutron coincidence counters. Gamma-ray assay methods have not been successful with some residues because of random lumps of plutonium metal. In this paper, we present measurements of MSE residues with two state-of-the-art neutron coincidence counters at the Los Alamos Plutonium Processing Facility: an in-line counter built for the assay of bulk waste material and the pyrochemical multiplicity counter that underwent test and evaluation at that facility. Both of these counters were designed to minimize the effects on measurements of variations in the sample geometry and variable energy spectra of emitted neutrons. These results are compared to measurements made with an HLNCII and with a 20-yr-old in-line well counter. The latter two counters are not optimized in ft sense. We conclude that the newer counters provide significantly improved assay results. The pyrochemical multiplicity counter operated in the conventional coincidence mode provided the best assays overall.

Book Energy Research Abstracts

Download or read book Energy Research Abstracts written by and published by . This book was released on 1995 with total page 782 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Radioactive Waste Management

Download or read book Radioactive Waste Management written by and published by . This book was released on 1981 with total page 536 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Government Reports Announcements   Index

Download or read book Government Reports Announcements Index written by and published by . This book was released on 1994 with total page 1500 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book ERDA Energy Research Abstracts

Download or read book ERDA Energy Research Abstracts written by and published by . This book was released on 1983 with total page 972 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Government reports annual index

Download or read book Government reports annual index written by and published by . This book was released on 199? with total page 1362 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Publications of the National Institute of Standards and Technology     Catalog

Download or read book Publications of the National Institute of Standards and Technology Catalog written by National Institute of Standards and Technology (U.S.) and published by . This book was released on 1981 with total page 680 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book NBS Special Publication

Download or read book NBS Special Publication written by and published by . This book was released on 1968 with total page 684 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Publications

Download or read book Publications written by United States. National Bureau of Standards and published by . This book was released on 1981 with total page 684 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Publications of the National Bureau of Standards     Catalog

Download or read book Publications of the National Bureau of Standards Catalog written by United States. National Bureau of Standards and published by . This book was released on 1980 with total page 686 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Test and Evaluation of the Dual range Coincidence Counter at the Savannah River Plant

Download or read book Test and Evaluation of the Dual range Coincidence Counter at the Savannah River Plant written by and published by . This book was released on 1981 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: This report describes the test and evaluation of a Los Alamos National Laboratory-designed dual-range neutron coincidence counter at the Savannah River Plant Separations Area. A variety of incoming plutonium metal and oxide shipments were assayed with the counter. Assay accuracies were 2% l sigma for pure metal, about 10% l sigma for impure metal, and 3% l sigma for oxide that was analyzed on a batch-by-batch basis.

Book Final Evaluation of Characterizing Pipe over pack Containers Using High Efficiency Neutron Counters

Download or read book Final Evaluation of Characterizing Pipe over pack Containers Using High Efficiency Neutron Counters written by and published by . This book was released on 2009 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Nondestructive assay (NDA) measurements of Transuranic (TRU) waste at Los Alamos National Laboratory (LANL) packed in Pipe-over-Pack Containers (POC) contain a number of complexities. The POC is highly attenuating to both gamma rays and neutrons which presents a difficult waste matrix for correct quantification of material in the container. Currently there are a number ofPOC containers at LANL that require evaluation for shipment to the Waste Isolation Pilot Plant (WIPP) in Carlsbad, NM. Updated data has been evaluated that finalizes the evaluation of characterizing Pipe-Over-Pack Containers. Currently at LANL, a single instrument has been used to explore the appropriateness of both passive neutron and quantitative gamma ray methods for measuring POC's. The passive neutron approach uses the Reals coincidence count rate to establish plutonium mass and other parameters of interest for TRU waste. The quantitative gamma ray method assumes a homogeneous distribution of radioactive source material with the surrounding material throughout the drum volume. Drums are assayed with a calibration based on the known density of the matrix. Both methods are supplemented by a simultaneous isotopic measurement using Multi-Group Analysis (MGA) to determine the plutonium isotopic composition. If MGA fails to provide a viable isotopic result Fixed Energy Response function Analysis with Multiple efficiencies (FRAM) has been used to replace the MGA results. Acceptable Knowledge (AK) may also be used in certain instances. This report will discuss the two methods in detail. Included in the discussion will be descriptions of the setup parameters and calibration techniques for the instrument. A number of test measurements have been performed to compare HENC data with certified historical data. Empty POCs loaded with known sources have also been measured to determine the viability of the technique. A comparison between calorimetry data, historical measurements and HENC data will also be performed. The conclusion will show that the current calibration on the HENC units is viable for analysis of POCs.

Book Transactions of the American Nuclear Society

Download or read book Transactions of the American Nuclear Society written by and published by . This book was released on 1987 with total page 96 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nuclear Science Abstracts

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1972 with total page 882 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Bulletin of the Atomic Scientists

Download or read book Bulletin of the Atomic Scientists written by and published by . This book was released on 1971-09 with total page 56 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Bulletin of the Atomic Scientists is the premier public resource on scientific and technological developments that impact global security. Founded by Manhattan Project Scientists, the Bulletin's iconic "Doomsday Clock" stimulates solutions for a safer world.

Book Scientific and Technical Aerospace Reports

Download or read book Scientific and Technical Aerospace Reports written by and published by . This book was released on 1970 with total page 340 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Transactions

Download or read book Transactions written by American Nuclear Society and published by . This book was released on 1987 with total page 1392 pages. Available in PDF, EPUB and Kindle. Book excerpt: