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Book Transmission Nuclear Resonance Fluorescence Measurements of 238U in Thick Targets

Download or read book Transmission Nuclear Resonance Fluorescence Measurements of 238U in Thick Targets written by and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Transmission nuclear resonance fluorescence measurements were made on targets consisting of Pb and depleted U with total areal densities near 86 g/cm2. The 238U content n the targets varied from 0 to 8.5percent (atom fraction). The experiment demonstrates the capability of using transmission measurements as a non-destructive technique to identify and quantify the presence of an isotope in samples with thicknesses comparable to he average thickness of a nuclear fuel assembly. The experimental data also appear to demonstrate the process of notch refilling with a predictable intensity. Comparison of measured spectra to previous backscatter 238U measurements indicates general agreement in observed excited states. Two new 238U excited states and possibly a third state have also been observed.

Book Nuclear Resonance Fluorescence for Nuclear Materials Assay

Download or read book Nuclear Resonance Fluorescence for Nuclear Materials Assay written by Brian Joseph Quiter and published by . This book was released on 2010 with total page 510 pages. Available in PDF, EPUB and Kindle. Book excerpt: This dissertation examines the measurement of nuclear resonance fluorescence gamma-rays as a technique to non-destructively determine isotopic compositions of target materials that are of interest for nuclear security applications. The physical processes that can result in non-resonant background to nuclear resonance fluorescence measurements are described and investigated using a radiation transport computer code that relies on the Monte Carlo technique, MCNPX. The phenomenon of nuclear resonance fluorescence is discussed with consideration of the angular distributions of resonance emissions, the effects of nuclear recoil, and the influence of thermal motion. Models describing two ways of measuring nuclear resonance fluorescence rates in materials are considered. First the measurement of back-scattered photons is considered. In this type of measurement, the portion of the interrogating photon beam that is scattered into large relative angles is measured. When the radioactivity of the target can be overcome by shielding or by use of intense photon sources, direct measurement of gamma-rays, emitted during nuclear resonance fluorescence can provide quantitative signatures that appear to be useful for applications such as forensic age-dating of large radiological sources. However, if the target radioactivity is too intense, as in the case for most spent nuclear fuel, a second measurement type, where indirect measurement of transmitted resonant-energy photons can also provide quantitative information. This method allows radiation detectors to be better-shielded from target radioactivity, but suffers from a slower accrual rate of statistical confidence. The models described herein indicate that very intense photon sources and large high-resolution detector arrays would be needed to measure 239Pu content in spent fuel to precisions desired by nuclear safeguards organizations. However, the rates at which statistics accrue are strongly proportional to the strengths of the resonances, and measurement of a plutonium isotope with stronger resonances may provide more practical measurement rates. The model for predicting relative detection rates of nuclear resonance fluorescence gamma-rays in the transmission measurement was experimentally tested using the 238U in a mixture of depleted uranium and lead as a surrogate for 239Pu in spent fuel. The experiment indicated that the model was approximately correct, but that the process of notch refilling, which was excluded from the initial model, appears to be visible. Data files of the computer code, MCNPX, were modified to allow for nuclear resonance fluorescence to be simulated and a bug in the code was repaired to allow the code to more accurately simulate non-resonant elastic photon scattering. Simulations using this modified version of MCNPX have indicated that the magnitude of the notch refill process is comparable to that of the difference between the analytical model and the experimental data.

Book Analytical Methods for Nonproliferation

Download or read book Analytical Methods for Nonproliferation written by Edward C. Morse and published by Springer. This book was released on 2016-04-04 with total page 254 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book is intended to be used as a textbook and research reference for the field of nuclear nonproliferation. The book is primarily technical and focussed on methods of detecting clandestine nuclear material that might be illicitly transported. The book also touches on nuclear forensics, i.e. methods for identification, attribution, and establishment of transport pathways for illicit nuclear material. Also covered are topics of methods used for arms control and treaty verification, and an assessment of technologies under development for all of the above. A description of the government and international agencies involved in nuclear terrorism prevention, nuclear safeguards, and arms control is also included.

Book Measurement and Resonance Analysis of Neutron Transmissions Through Four Samples of 238U

Download or read book Measurement and Resonance Analysis of Neutron Transmissions Through Four Samples of 238U written by and published by . This book was released on 1977 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Accurate total and partial cross sections for 238U are important for nuclear reactor design. In the resolved resonance region, energies below 4.0 keV, these cross sections are described in terms of individual resonance parameters of which the neutron widths in the 1.5 to 4.0 keV region from various workers appear discrepant. In order to determine these widths, (0.880 to 100.0 keV) neutron transmissions through 0.076, 0.254, 1.080, and 3.620 cm thick enriched 238U samples were measured, and (0.880 to 100.0 keV) range transmissions were analyzed. (GHT).

Book Passive Nondestructive Assay of Nuclear Materials

Download or read book Passive Nondestructive Assay of Nuclear Materials written by Doug Reilly and published by . This book was released on 1991 with total page 700 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book NBS Special Publication

Download or read book NBS Special Publication written by and published by . This book was released on 1968 with total page 684 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Energy Research Abstracts

Download or read book Energy Research Abstracts written by and published by . This book was released on 1986 with total page 876 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nuclear Resonance Fluorescence in Si28

Download or read book Nuclear Resonance Fluorescence in Si28 written by Jean L. Ryan and published by . This book was released on 1963 with total page 78 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Physics Briefs

Download or read book Physics Briefs written by and published by . This book was released on 1989-07 with total page 1314 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Publications of the National Institute of Standards and Technology     Catalog

Download or read book Publications of the National Institute of Standards and Technology Catalog written by National Institute of Standards and Technology (U.S.) and published by . This book was released on 1981 with total page 680 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Publications

Download or read book Publications written by United States. National Bureau of Standards and published by . This book was released on 1981 with total page 684 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book INIS Atomindex

Download or read book INIS Atomindex written by and published by . This book was released on 1985 with total page 1514 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nuclear Science Abstracts

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1973 with total page 1142 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Scientific and Technical Aerospace Reports

Download or read book Scientific and Technical Aerospace Reports written by and published by . This book was released on 1991 with total page 910 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Energy Research Abstracts

Download or read book Energy Research Abstracts written by and published by . This book was released on 1984 with total page 632 pages. Available in PDF, EPUB and Kindle. Book excerpt: Includes all works deriving from DOE, other related government-sponsored information and foreign nonnuclear information.