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Book Measurement of Plutonium in Spent Nuclear Fuel by Self induced X ray Fluorescence

Download or read book Measurement of Plutonium in Spent Nuclear Fuel by Self induced X ray Fluorescence written by and published by . This book was released on 2009 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Direct measurement of the plutonium content in spent nuclear fuel is a challenging problem in non-destructive assay. The very high gamma-ray flux from fission product isotopes overwhelms the weaker gamma-ray emissions from plutonium and uranium, making passive gamma-ray measurements impossible. However, the intense fission product radiation is effective at exciting plutonium and uranium atoms, resulting in subsequent fluorescence X-ray emission. K-shell X-rays in the 100 keV energy range can escape the fuel and cladding, providing a direct signal from uranium and plutonium that can be measured with a standard germanium detector. The measured plutonium to uranium elemental ratio can be used to compute the plutonium content of the fuel. The technique can potentially provide a passive, non-destructive assay tool for determining plutonium content in spent fuel. In this paper, we discuss recent non-destructive measurements of plutonium X-ray fluorescence (XRF) signatures from pressurized water reactor spent fuel rods. We also discuss how emerging new technologies, like very high energy resolution microcalorimeter detectors, might be applied to XRF measurements.

Book Un dernier mot sur l amortissement

Download or read book Un dernier mot sur l amortissement written by and published by . This book was released on with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Energy Research Abstracts

Download or read book Energy Research Abstracts written by and published by . This book was released on 1988 with total page 752 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nondestructive  Energy dispersive  X ray Fluorescence Analysis of Product Stream Concentrations from Reprocessed Nuclear Fuels

Download or read book Nondestructive Energy dispersive X ray Fluorescence Analysis of Product Stream Concentrations from Reprocessed Nuclear Fuels written by and published by . This book was released on 1979 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Energy-dispersive x-ray fluorescence analysis (XRFA) can be used to measure nondestructively pure and mixed U/Pu concentrations in process streams and hold tank solutions. The 122-keV gamma ray from 57Co excites the actinide K x rays which are detected by a HPGe detector. A computer- and disk-based analyzer system provides capability for making on-stream analyses, and the noninvasive measurement is easily adapted directly to appropriate sized pipes used in a chemical reprocessing plant. Measurement times depend on concentration and purpose but vary from 100 to 500s for process control of strong to weak solutions. Accountability measurements require better accuracy thus more time; and for solutions containing plutonium, require a measurement of the solution radioactivity made with an automatic shutter that eclipses the two exciting sources. Plutonium isotopic abundances can also be obtained. Concentrations in single or dual element solutions from less than 1 g/l to over 200 g/l are determined to an accuracy of 0.2% after calibration of the system. For mixed solutions the unknown ratio of U to Pu is linearly related to the net U/Pu K x-ray intensities. Concentration values for ratios different than the calibration ratio require only small corrections to the values derived from a calibration polynomial. Minor fission product contamination does not prevent concentration determinations by XRFA. The computer-based system also allows real-time dynamic concentration measurements to be made.

Book Transmission corrected X ray Fluorescence Analysis of Uranium and Plutonium Solutions Using a Dual Transmission Source

Download or read book Transmission corrected X ray Fluorescence Analysis of Uranium and Plutonium Solutions Using a Dual Transmission Source written by and published by . This book was released on 1987 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The energy-dispersive x-ray fluorescence analysis (XRFA) technique has been implemented at several spent nuclear fuel reprocessing facilities for nondestructive measurements of uranium and/or plutonium concentrations in process streams and product storage tanks. An important factor in these quantitative measurements is the absorption of the fluoresced x-rays by the solution matrix, which must be taken into account to accurately quantify the U or Pu concentrations. We describe a new, accurate method using a dual transmission source of Gd-153 and Co-57 to correct for matrix effects. Results of measurements on uranium and plutonium solution standards show the methodology to be better than 0.5%, which includes statistical precision, over the concentration range from 1 to 250 g/l. 5 refs., 4 figs., 3 tabs.

Book Passive Nondestructive Assay of Nuclear Materials

Download or read book Passive Nondestructive Assay of Nuclear Materials written by Doug Reilly and published by . This book was released on 1991 with total page 700 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nuclear Science Abstracts

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1976 with total page 934 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Scientific and Technical Aerospace Reports

Download or read book Scientific and Technical Aerospace Reports written by and published by . This book was released on 1971 with total page 284 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book INIS Atomindex

Download or read book INIS Atomindex written by and published by . This book was released on 1987 with total page 480 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Standard Test Method for Determination of Uranium and Plutonium Concentration in Aqueous Solutions Using Hybrid K Edge Densitometry and X Ray Fluorescence

Download or read book Standard Test Method for Determination of Uranium and Plutonium Concentration in Aqueous Solutions Using Hybrid K Edge Densitometry and X Ray Fluorescence written by and published by . This book was released on with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Determination of Uranium and Neptunium in Plutonium by X ray Fluorescence

Download or read book Determination of Uranium and Neptunium in Plutonium by X ray Fluorescence written by Calvin J. Martell and published by . This book was released on 1978 with total page 5 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Nuclear Science Abstracts

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1973 with total page 1162 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Transplutonium Elements

Download or read book Transplutonium Elements written by Charles E. Stuber and published by . This book was released on 1972 with total page 146 pages. Available in PDF, EPUB and Kindle. Book excerpt: