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Book Initial Results from Dissolution Rate Testing of N Reactor Spent Fuel Over a Range of Potential Geologic Repository Aqueous Conditions

Download or read book Initial Results from Dissolution Rate Testing of N Reactor Spent Fuel Over a Range of Potential Geologic Repository Aqueous Conditions written by and published by . This book was released on 1998 with total page 63 pages. Available in PDF, EPUB and Kindle. Book excerpt: Hanford N-Reactor spent nuclear fuel (HSNF) may ultimately be placed in a geologic repository for permanent disposal. To determine whether the engineered barrier system that will be designed for emplacement of light-water-reactor (LWR) spent fuel will also suffice for HSNF, aqueous dissolution rate measurements were conducted on the HSNF. The purpose of these tests was to determine whether HSNF dissolves faster or slower than LWR spent fuel under some limited repository-relevant water chemistry conditions. The tests were conducted using a flowthrough method that allows the dissolution rate of the uranium matrix to be measured without interference by secondary precipitation reactions that would confuse interpretation of the results. Similar tests had been conducted earlier with LWR spent fuel, thereby allowing direct comparisons. Two distinct corrosion modes were observed during the course of these 12 tests. The first, Stage 1, involved no visible corrosion of the test specimen and produced no undissolved corrosion products. The second, Stage 2, resulted in both visible corrosion of the test specimen and left behind undissolved corrosion products. During Stage 1, the rate of dissolution could be readily determined because the dissolved uranium and associated fission products remained in solution where they could be quantitatively analyzed. The measured rates were much faster than has been observed for LWR spent fuel under all conditions tested to date when normalized to the exposed test specimen surface areas. Application of these results to repository conditions, however, requires some comparison of the physical conditions of the different fuels. The surface area of LWR fuel that could potentially be exposed to repository groundwater is estimated to be approximately 100 times greater than HSNF. Therefore, when compared on the basis of mass, which is more relevant to repository conditions, the HSNF and LWR spent fuel dissolve at similar rates.

Book Proceedings of the Embedded Topical Meeting on DOE Spent Nuclear Fuel and Fissile Material Management  San Diego  California  June 4 8  2000

Download or read book Proceedings of the Embedded Topical Meeting on DOE Spent Nuclear Fuel and Fissile Material Management San Diego California June 4 8 2000 written by and published by . This book was released on 2000 with total page 556 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Proceedings of the Third Topical Meeting on DOE Spent Nuclear Fuel and Fissile Materials Management

Download or read book Proceedings of the Third Topical Meeting on DOE Spent Nuclear Fuel and Fissile Materials Management written by American Nuclear Society and published by . This book was released on 1998 with total page 454 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Summary of Results from the Series 2 and Series 3 NNWSI Bare Fuel Dissolution Tests

Download or read book Summary of Results from the Series 2 and Series 3 NNWSI Bare Fuel Dissolution Tests written by Charles N. Wilson and published by . This book was released on 1987 with total page 15 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Nevada Nuclear Waste Storage Investigations (NNWSI) Project is studying dissolution and radionuclide release behavior of spent nuclear fuel in Nevada Test Site groundwater. Specimens were tested for multiple cycles in J-13 well water. The Series 2 tests were run in unsealed silica vessels under ambient hot cell air (25°C) for five cycles for a total of 34 months. The Series 3 tests were run in sealed stainless steel vessels at 25°C and 85°C for three cycles for a total of 15 months. Selected summary results from Series 2 and Series 3 tests with bare fuel specimens are reported. Uranium concentrations in later test cycles ranged from 1 to 2 [mu]g/ml in the Series 2 Tests versus about 0.1 to 0.4 [mu]g/ml in Series 3 with the lowest concentrations occurring in the 85°C tests. Preferential release of fission products Cs, I, Sr and Tc, and activation product C-14, was indicated relative to the actinides. Tc-99 and Cs-137 activities measured in solution after Cycle 1 increased linearly with time, with the rate of increase greater at 85°C than at 25°C.

Book Advances in High Temperature Gas Cooled Reactor Fuel Technology

Download or read book Advances in High Temperature Gas Cooled Reactor Fuel Technology written by International Atomic Energy Agency and published by . This book was released on 2012-06 with total page 639 pages. Available in PDF, EPUB and Kindle. Book excerpt: This publication reports on the results of a coordinated research project on advances in high temperature gas cooled reactor (HTGR) fuel technology and describes the findings of research activities on coated particle developments. These comprise two specific benchmark exercises with the application of HTGR fuel performance and fission product release codes, which helped compare the quality and validity of the computer models against experimental data. The project participants also examined techniques for fuel characterization and advanced quality assessment/quality control. The key exercise included a round-robin experimental study on the measurements of fuel kernel and particle coating properties of recent Korean, South African and US coated particle productions applying the respective qualification measures of each participating Member State. The summary report documents the results and conclusions achieved by the project and underlines the added value to contemporary knowledge on HTGR fuel.

Book Nuclear Wastes

    Book Details:
  • Author : National Research Council
  • Publisher : National Academies Press
  • Release : 1996-02-23
  • ISBN : 0309052262
  • Pages : 590 pages

Download or read book Nuclear Wastes written by National Research Council and published by National Academies Press. This book was released on 1996-02-23 with total page 590 pages. Available in PDF, EPUB and Kindle. Book excerpt: Disposal of radioactive waste from nuclear weapons production and power generation has caused public outcry and political consternation. Nuclear Wastes presents a critical review of some waste management and disposal alternatives to the current national policy of direct disposal of light water reactor spent fuel. The book offers clearcut conclusions for what the nation should do today and what solutions should be explored for tomorrow. The committee examines the currently used "once-through" fuel cycle versus different alternatives of separations and transmutation technology systems, by which hazardous radionuclides are converted to nuclides that are either stable or radioactive with short half-lives. The volume provides detailed findings and conclusions about the status and feasibility of plutonium extraction and more advanced separations technologies, as well as three principal transmutation concepts for commercial reactor spent fuel. The book discusses nuclear proliferation; the U.S. nuclear regulatory structure; issues of health, safety and transportation; the proposed sale of electrical energy as a means of paying for the transmutation system; and other key issues.

Book Radioactive Waste Management

Download or read book Radioactive Waste Management written by and published by . This book was released on 1981 with total page 622 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Results from Nevada Nuclear Waste Storage Investigations  NNWSI  Series 3 Spent Fuel Dissolution Tests

Download or read book Results from Nevada Nuclear Waste Storage Investigations NNWSI Series 3 Spent Fuel Dissolution Tests written by and published by . This book was released on 2001 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The dissolution and radionuclide release behavior of spent fuel in groundwater is being studied by the Yucca Mountain Project (YMP), formerly the Nevada Nuclear Waste Storage Investigations (NNWSI) Project. Specimens prepared from pressurized water reactor fuel rod segments were tested in sealed stainless steel vessels in Nevada Test Site J-13 well water at 85[degree]C and 25[degree]C. The test matrix included three specimens of bare-fuel particles plus cladding hulls, two fuel rod segments with artificially defected cladding and water-tight end fittings, and an undefected fuel rod section with watertight end fittings. Periodic solution samples were taken during test cycles with the sample volumes replenished with fresh J-13 water. Test cycles were periodically terminated and the specimens restarted in fresh J-13 water. The specimens were run for three cycles for a total test duration of 15 months. 22 refs., 32 figs., 26 tabs.

Book Radioactive Waste Forms for the Future

Download or read book Radioactive Waste Forms for the Future written by Werner Lutze and published by North Holland. This book was released on 1988 with total page 802 pages. Available in PDF, EPUB and Kindle. Book excerpt: This volume presents a compilation of important information on the full range of radioactive waste forms that have been developed, or at least suggested, for the incorporation of high-level nuclear waste. Many of the results were published in the ''gray literature'' of final reports of national laboratories or in various, generally less available, proceedings volumes. This is the first publication to draw information on nuclear waste forms for high-level wastes together into a single volume. Although borosilicate glass has become the standard waste form, additional research in this compound is still necessary. With improved technology (particularly processing technologies) and with a more detailed knowledge of repository conditions, glasses and second generation waste forms with improved performance properties can be developed. Sustained research programs on nuclear waste form development will yield results that can only add to public confidence and the final, safe disposal of nuclear waste. The aim of this volume is to provide a 'spring board' for these future research efforts. A detailed presentation is given on the properties and performance of non-crystalline waste forms (borosilicate glass, sintered glass, and lead-iron phosphate glass), and crystalline waste forms (Synroc, tailored ceramics, TiO 2 - ceramic matrix, glass-ceramics and FUETAP concrete). A chapter on Novel Waste Forms reviews a number of methods that warrant further development because of their potential superior performance and unique applications. The final chapter includes a tabulated comparison of important waste form properties and an extended discussion on the corrosion process and radiation damage effects for each waste form. Of particular interest is a performance assessment of nuclear waste borosilicate glass and the crystalline ceramic Synroc. This is the first detailed attempt to compare these two important waste forms on the basis of their materials properties. The discussion emphasizes the difficulties in making such a comparison and details the types of data that are required. Each chapter has been written by an expert and includes a current compilation of waste form properties with an extensive list of references. This volume will provide a stimulus for future research as well as useful reference material for scientists working in the field of nuclear waste disposal and materials science.

Book Energy  Waste and the Environment

Download or read book Energy Waste and the Environment written by R. Gieré and published by Geological Society of London. This book was released on 2004 with total page 694 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book provides incentives for further development of sustainable fuel cycles through a novel and interdisciplinary approach to an Earth science-related topic. The main focus is on geochemical concepts in immobilizing, isolating or neutralizing waste derived from energy production and consumption. The book also addresses the issue of using some types of energy-derived waste as alternative raw materials. Moreover, it highlights research on how certain wastes can be used for energy production, an increasingly important aspect of modern integrated waste management strategies. The main objectives are to: (a) identify the most serious environmental problems related to various types of power generation and associated waste accumulation; (b) present strategies, based on natural analogue materials, for the immobilization of toxic and radioactive waste components through mineralogical barriers; (c) discuss modern procedures for reuse of waste or certain waste components; and (d) review the importance of geochemical modelling in describing and predicting the interaction between waste and the environment.

Book Spent fuel Test Climax

Download or read book Spent fuel Test Climax written by W. C. Patrick and published by . This book was released on 1986 with total page 19 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Strategy and Methodology for Radioactive Waste Characterization

Download or read book Strategy and Methodology for Radioactive Waste Characterization written by International Atomic Energy Agency and published by IAEA. This book was released on 2007 with total page 188 pages. Available in PDF, EPUB and Kindle. Book excerpt: Over the past decade significant progress has been achieved in the development of waste characterization and control procedures and equipment as a direct response to ever-increasing requirements for quality and reliability of information on waste characteristics. Failure in control procedures at any step can have important, adverse consequences and may result in producing waste packages which are not compliant with the waste acceptance criteria for disposal, thereby adversely impacting the repository. The information and guidance included in this publication corresponds to recent achievements and reflects the optimum approaches, thereby reducing the potential for error and enhancing the quality of the end product. -- Publisher's description.

Book Ceramic Abstracts

    Book Details:
  • Author : American Ceramic Society
  • Publisher :
  • Release : 1993
  • ISBN :
  • Pages : 1252 pages

Download or read book Ceramic Abstracts written by American Ceramic Society and published by . This book was released on 1993 with total page 1252 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book State of the art Report on the Progress of Nuclear Fuel Cycle Chemistry

Download or read book State of the art Report on the Progress of Nuclear Fuel Cycle Chemistry written by and published by . This book was released on 2018 with total page 148 pages. Available in PDF, EPUB and Kindle. Book excerpt: The implementation of advanced nuclear systems requires that new technologies associated with the back end of the fuel cycle are developed. The separation of minor actinides from other fuel components is one of the advanced concepts being studied to help close the nuclear fuel cycle and to improve the long-term effects on the performance of geological repositories. Separating spent fuel elements and subsequently converting them through transmutation into short-lived nuclides should considerably reduce the longterm risks associated with nuclear power generation.

Book Energy Research Abstracts

Download or read book Energy Research Abstracts written by and published by . This book was released on 1990 with total page 498 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Hydrolysis of Metal Ions

    Book Details:
  • Author : Paul L. Brown
  • Publisher : John Wiley & Sons
  • Release : 2016-02-23
  • ISBN : 3527656200
  • Pages : 1449 pages

Download or read book Hydrolysis of Metal Ions written by Paul L. Brown and published by John Wiley & Sons. This book was released on 2016-02-23 with total page 1449 pages. Available in PDF, EPUB and Kindle. Book excerpt: Endlich ein Fachbuch, das die Theorie, Methoden und die verschiedenen Arten von Metall-Ionen-Komplexen in Wasser (Hydrolyse) umfassend behandelt. Geschrieben wurde dieses Referenzwerk von einem Kernchemiker aus dem Hochschulbereich und einem Geochemiker aus der Industrie. Behandelt werden Kationen- und Anionen-Komplexe sowie die Metall-Ionen-Hydrolyse, zu der zunächst Hintergrundinformationen geliefert werden, bevor eine Beschreibung der Dissoziation von Wasser, aller verschiedenen Hydrolysekomplexe und Verbindungen von Metall und Wasser folgt. Ein Muss für Wissenschaftler im universitären Umfeld und in der Industrie, die sich mit diesem interdisziplinären Thema beschäftigen.