Download or read book Distribution and Direct Radiative Forcing of Carbonaceous and Sulfate Aerosols in an Interactive Size resolving Aerosol climate Model written by Dongchul Kim and published by . This book was released on 2008 with total page 36 pages. Available in PDF, EPUB and Kindle. Book excerpt: A multimode, two-moment aerosol model has been incorporated in the NCAR CAM3 to develop an interactive aerosol-climate model and to study the impact of anthropogenic aerosols on the global climate system. Currently, seven aerosol modes, namely three for external sulfate, one each for external black carbon (BC), external organic carbon (OC), sulfate/BC mixture (MBS; with BC core coated by sulfate shell), and sulfate/OC mixture (MOS; a uniform mixture of OC and sulfate) are included in the model. Both mass and number concentrations of each aerosol mode as well as the mass of carbonaceous species in the mixed modes are predicted by the model so that the chemical, physical, and radiative processes of various aerosols can be formulated depending on aerosol's size, chemical composition, and mixing state. Comparisons of modeled surface and vertical aerosol concentrations as well as the optical depth of aerosols with available observations and previous model estimates are in general agreement. However, some discrepancies do exist likely caused by the coarse model resolution or the constant rates of anthropogenic emissions used to test the model. Comparing to the widely used mass-only method with prescribed geometric size of particles (one-moment scheme), the use of prognostic size distributions of aerosols based on a two-moment scheme in our model leads to a significant reduction in optical depth and thus the radiative forcing at the top of the atmosphere (TOA) of particularly external sulfate aerosols. The inclusion of two types of mixed aerosols alters the mass partitioning of carbonaceous and sulfate aerosol constituents: about 35.5%, 48.5%, and 32.2% of BC, OC, and sulfate mass are found in the mixed aerosols. This also brings in competing effects in aerosol radiative forcing including a reduction in atmospheric abundance of BC and OC due to the shorter lifetime of internal mixtures (cooling), a mass loss of external sulfate to mixtures (warming), and an enhancement in atmospheric heating per BC mass due to the stronger absorption extinction of the MBS than external BC (warming). The combined result of including a prognostic size distribution and the mixed aerosols in the model is a much smaller total negative TOA forcing (-0.12 Wm-2) of all carbonaceous and sulfate aerosol compounds compared to the cases using one-moment scheme either excluding or including internal mixtures (-0.42 and -0.71 W-2, respectively). In addition, the global mean all-sky TOA direct forcing of aerosols is significantly more positive than the clear-sky value due to the existence of low clouds beneath the absorbing (external BC and MBS) aerosol layer, particularly over a dark surface. An emission reduction of about 44% for BC and 38% of primary OC is found to effectively change the TOA radiative forcing of the entire aerosol family by -0.14 Wm-2 for clear-sky and -0.29 Wm-2 for all-sky.
Download or read book A Plan for a Research Program on Aerosol Radiative Forcing and Climate Change written by Panel on Aerosol Radiative Forcing and Climate Change and published by National Academies Press. This book was released on 1996-05-01 with total page 180 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book recommends the initiation of an "integrated" research program to study the role of aerosols in the predicted global climate change. Current understanding suggest that, even now, aerosols, primarily from anthropogenic sources, may be reducing the rate of warming caused by greenhouse gas emissions. In addition to specific research recommendations, this book forcefully argues for two kinds of research program integration: integration of the individual laboratory, field, and theoretical research activities and an integrated management structure that involves all of the concerned federal agencies.
Download or read book High Resolution Aerosol Modeling written by and published by . This book was released on 2005 with total page 3 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Atmospheric Science Division of LLNL has performed high-resolution calculations of direct sulfate forcing using a DOE-provided computer resource at NERSC. We integrated our global chemistry-aerosol model (IMPACT) with the LLNL high-resolution global climate model (horizontal resolution as high as 100 km) to examine the temporal evolution of sulfate forcing since 1950. We note that all previous assessments of sulfate forcing reported in IPCC (2001) were based on global models with coarse spatial resolutions ((almost equal to) 300 km or even coarser). However, the short lifetime of aerosols ((almost equal to) days) results in large spatial and temporal variations of radiative forcing by sulfate. As a result, global climate models with coarse resolutions do not accurately simulate sulfate forcing on regional scales. It requires much finer spatial resolutions in order to address the effects of regional anthropogenic SO2 emissions on the global atmosphere as well as the effects of long-range transport of sulfate aerosols on the regional climate forcing. By taking advantage of the tera-scale computer resources at NERSC, we simulated the historic direct sulfate forcing at much finer spatial resolutions than ever attempted before. Furthermore, we performed high-resolution chemistry simulations and saved monthly averaged oxidant fields, which will be used in subsequent simulations of sulfate aerosol formation and their radiative impact.
Download or read book The Direct Radiative Forcing Effects of Aerosols on the Climate in California written by Hui Du and published by . This book was released on 2009 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The Weather Research and Forecast (WRF) model is used to explore the influence of aerosol direct radiative effects on regional climate of California. Aerosol data is provided by the MOZART global chemistry transport model and includes sulfate, black carbon, organic carbon, dust and sea salt. To investigate the sensitivity of aerosol radiative effects to different aerosol species and to the quantity of sulfate and dust, tests are conducted by using different combinations of aerosols and by resetting the quantity of sulfate and dust. The model results show that all the considered aerosols could have a cooling effect of one half to one degree in terms of temperature and that dust and sulfate are the most important aerosols. However, large uncertainties exist. The results suggest that the dust from MOZART is greatly overestimated over the simulation domain. The single scattering albedo (SSA) values of dust used in some global climate models are likely underestimated compared to recent studies on dust optical properties and could result in overestimating the corresponding cooling effects by approximately 0.1 degree. Large uncertainties exist in estimating the roles of different forcing factors which are causing the observed temperature change in the past century in California.
Download or read book Impact of Sulfur and Carbonaceous Emissions from International Shipping on Aerosol Distributions and Direct Radiative Forcing written by Chien Wang (Atmospheric Chemistry Research Scientist.) and published by . This book was released on 2008 with total page 8 pages. Available in PDF, EPUB and Kindle. Book excerpt: We describe in this report an effort using the MIT/NCAR three-dimensional aerosol-climate model to study the impact of ship emissions on chemical composition and radiative forcing of aerosols. Our results indicate that international shipping can be a non-negligible factor in determining the radiative forcing of aerosols over specific regions with intensive ship activities. These places include the European, eastern Asian, and American coastal regions. The global mean aerosol radiative forcing caused by the ship emissions ranges from -12.5 to -23 mW/m2, depending on whether the mixing between black carbon and sulfate is included in the model. However, over the aforementioned places, the radiative forcing resulting from ship emissions can be much more important in the total regional aerosol forcing.
Download or read book Radiative Forcing of Climate Change written by National Research Council and published by National Academies Press. This book was released on 2005-03-25 with total page 222 pages. Available in PDF, EPUB and Kindle. Book excerpt: Changes in climate are driven by natural and human-induced perturbations of the Earth's energy balance. These climate drivers or "forcings" include variations in greenhouse gases, aerosols, land use, and the amount of energy Earth receives from the Sun. Although climate throughout Earth's history has varied from "snowball" conditions with global ice cover to "hothouse" conditions when glaciers all but disappeared, the climate over the past 10,000 years has been remarkably stable and favorable to human civilization. Increasing evidence points to a large human impact on global climate over the past century. The report reviews current knowledge of climate forcings and recommends critical research needed to improve understanding. Whereas emphasis to date has been on how these climate forcings affect global mean temperature, the report finds that regional variation and climate impacts other than temperature deserve increased attention.
Download or read book Climate Change 2013 The Physical Science Basis written by Intergovernmental Panel on Climate Change (IPCC) and published by Cambridge University Press. This book was released on 2014-03-24 with total page 1554 pages. Available in PDF, EPUB and Kindle. Book excerpt: This Fifth Assessment Report of the Intergovernmental Panel on Climate Change (IPCC) will again form the standard scientific reference for all those concerned with climate change and its consequences, including students and researchers in environmental science, meteorology, climatology, biology, ecology and atmospheric chemistry. It provides invaluable material for decision makers and stakeholders at international, national and local level, in government, businesses, and NGOs. This volume provides: • An authoritative and unbiased overview of the physical science basis of climate change • A more extensive assessment of changes observed throughout the climate system than ever before • New dedicated chapters on sea-level change, biogeochemical cycles, clouds and aerosols, and regional climate phenomena • Extensive coverage of model projections, both near-term and long-term climate projections • A detailed assessment of climate change observations, modelling, and attribution for every continent • A new comprehensive atlas of global and regional climate projections for 35 regions of the world
Download or read book Mixed Phase Clouds written by Constantin Andronache and published by Elsevier. This book was released on 2017-09-28 with total page 302 pages. Available in PDF, EPUB and Kindle. Book excerpt: Mixed-Phase Clouds: Observations and Modeling presents advanced research topics on mixed-phase clouds. As the societal impacts of extreme weather and its forecasting grow, there is a continuous need to refine atmospheric observations, techniques and numerical models. Understanding the role of clouds in the atmosphere is increasingly vital for current applications, such as prediction and prevention of aircraft icing, weather modification, and the assessment of the effects of cloud phase partition in climate models. This book provides the essential information needed to address these problems with a focus on current observations, simulations and applications. - Provides in-depth knowledge and simulation of mixed-phase clouds over many regions of Earth, explaining their role in weather and climate - Features current research examples and case studies, including those on advanced research methods from authors with experience in both academia and the industry - Discusses the latest advances in this subject area, providing the reader with access to best practices for remote sensing and numerical modeling
Download or read book Climate Implications of Carbonaceous Aerosols written by and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Recently, attention has been drawn towards black carbon aerosols as a likely short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and its climate interactions. Black carbon is directly released as particle into the atmosphere, but then interacts with other gases and particles through condensation and coagulation processes leading to further aerosol growth, aging and internal mixing. A detailed aerosol microphysical scheme, MATRIX, embedded within the global GISS modelE includes the above processes that determine the lifecycle and climate impact of aerosols. This study presents a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing change is -0.56 W/m2 between 1750 and 2000. However, the direct and indirect aerosol effects are very sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties. Assuming that sulfates, nitrates and secondary organics form a coating shell around a black carbon core, rather than forming a uniformly mixed particles, changes the overall net radiative forcing from a negative to a positive number. Black carbon mitigation scenarios showed generally a benefit when mainly black carbon sources such as diesel emissions are reduced, reducing organic and black carbon sources such as bio-fuels, does not lead to reduced warming.
Download or read book Aerosol Cloud Interactions from Urban Regional to Global Scales written by Yuan Wang and published by Springer. This book was released on 2015-05-05 with total page 100 pages. Available in PDF, EPUB and Kindle. Book excerpt: The studies in this dissertation aim at advancing our scientific understandings about physical processes involved in the aerosol-cloud-precipitation interaction and quantitatively assessing the impacts of aerosols on the cloud systems with diverse scales over the globe on the basis of the observational data analysis and various modeling studies. As recognized in the Fifth Assessment Report by the Inter-government Panel on Climate Change, the magnitude of radiative forcing by atmospheric aerosols is highly uncertain, representing the largest uncertainty in projections of future climate by anthropogenic activities. By using a newly implemented cloud microphysical scheme in the cloud-resolving model, the thesis assesses aerosol-cloud interaction for distinct weather systems, ranging from individual cumulus to mesoscale convective systems. This thesis also introduces a novel hierarchical modeling approach that solves a long outstanding mismatch between simulations by regional weather models and global climate models in the climate modeling community. More importantly, the thesis provides key scientific solutions to several challenging questions in climate science, including the global impacts of the Asian pollution. As scientists wrestle with the complexities of climate change in response to varied anthropogenic forcing, perhaps no problem is more challenging than the understanding of the impacts of atmospheric aerosols from air pollution on clouds and the global circulation.
Download or read book Observing and Modeling Earth s Energy Flows written by Lennart Bengtsson and published by Springer. This book was released on 2012-09-07 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book provides a comprehensive presentation of Earth’s energy flows and their consequences for the climate. The Earth’s climate as well as planetary climates in general, are broadly controlled by three fundamental parameters: the solar irradiance, the planetary albedo and the planetary emissivity. Space measurements indicate that these three quantities are remarkably stable. A minor decrease in planetary emissivity is consistent with theoretical calculations. This is due to the ongoing increase of atmospheric greenhouse gases making the atmosphere more opaque to long wave terrestrial radiation. As a consequence radiation processes are slightly out of balance as less heat is leaving the Earth in the form of thermal radiation than the incoming amount of heat from the sun. Present space-based systems cannot yet satisfactorily measure this imbalance, but the effect can be inferred from the measurements of the increase of heat in the oceans. Minor amounts of heat are also used to melt ice and to warm the atmosphere and the surface of the Earth. The book brings to fore the complexity of feedback processes of the Earth’s climate system and in particular the way clouds and aerosols affect the energy balance both directly and indirectly through feed-back loops driven by the dynamics of atmospheric, ocean and land surface processes. The book highlights recent scientific progress as well as remaining challenges. Previously published in Surveys in Geophysics, Volume 33, Nos. 3-4, 2012
Download or read book Climate Change 2013 The Physical Science Basis written by Intergouvernemental panel on climate change. Working group 1 and published by Cambridge University Press. This book was released on 2014 with total page 1553 pages. Available in PDF, EPUB and Kindle. Book excerpt: The report also provides a comprehensive assessment of past and future sea level change in a dedicated chapter.
Download or read book Atmospheric Aerosol Properties and Climate Impacts written by and published by . This book was released on 2009 with total page 128 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Atmospheric Aerosol Properties and Climate Impacts written by and published by . This book was released on 2009 with total page 136 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Aerosol Forcing of Climate written by R. J. Charlson and published by . This book was released on 1995-08-24 with total page 460 pages. Available in PDF, EPUB and Kindle. Book excerpt: Global climate change as a consequence of anthropogenic changes in the chemical composition of the atmosphere poses scientific questions of a nature and interdisciplinary scope that are unprecedented. Uncertainties in the climate forecast are large and thus far have hampered the establishment of a clear world plan for preventing or mitigating against unacceptable effects. The forecast of global and regional climate changes depends upon the development of a sound understanding of the factors that change the global heat balance and thus influence the climate. Changes in heat balance due to anthropogenic or externally imposed changes in the chemical composition of the atmosphere are referred to as forcings. While the uncertainties in the global mean greenhouse-gas forcing are not negligible (??? 15%), uncertainties in forcings by changes in the atmospheric aerosol and in clouds are much larger, and in some cases even include uncertainty in the sign of the forcing. Reductionist science, with its compartmentalized disciplines, has not coped effectively with the scientific problems of aerosols and their effects, largely because of a need for simultaneous consideration of chemical processes, chemical properties, physical properties, and a wide variety of physical processes and consequences. In the case of natural aerosols and their effects on clouds, it is even necessary to include studies of microbiology and of biochemistry. This volume ? the record of intense, interdisciplinary debate between atmospheric chemists, meteorologists, physicists, and biogeochemists - considers the subset of climate forcings due to atmospheric aerosols, with particular emphasis on integrating the necessary disciplinary components. It is truly unique in its interdisciplinary approach. The information contained in the overview papers and summary reports will be of interest to policymakers and scientists alike. Goal of this Dahlem Workshop to assess the controlling factors, geographic and temporal variations of the radiative properties of atmospheric aerosols, and to examine the extent to which their forcing through direct and indirect effects counteracts greenhouse-gas forcing on regional and global climate.
Download or read book Aerosol Effects on Climate written by S. G. Jennings and published by University of Arizona Press. This book was released on 1993-01-01 with total page 324 pages. Available in PDF, EPUB and Kindle. Book excerpt: There is now a growing awareness that, in addition to the well publicized influence of carbon dioxide and other greenhouse gases on the warming of the earth's atmosphere, aerosol particles may also play an important role in forcing climate change. This volume brings together previously unavailable data and interpretative analyses, derived from studies in both the U.S. and U.S.S.R., which review, update, and assess aerosol-related climatic effects.
Download or read book Atmospheric Aerosol Properties and Climate Impacts written by Mian Chin and published by DIANE Publishing. This book was released on 2009-05 with total page 128 pages. Available in PDF, EPUB and Kindle. Book excerpt: This Synthesis and Assessment Product (SAP) critically reviews current knowledge about global distributions and properties of atmospheric aerosols, as they relate to aerosol impacts on climate. It assesses possible next steps aimed at substantially reducing uncertainties in aerosol radiative forcing estimates. Current measurement techniques and modeling approaches are summarized, providing context. The objectives of this report are: (1) to promote a consensus about the knowledge base for climate change decision support; and (2) to provide a synthesis and integration of the current knowledge of the climate-relevant impacts of anthropogenic aerosols. Illustrations.
