Download or read book Ultrafast Dynamics in Helium Nanodroplets Probed by Femtosecond Time resolved EUV Photoelectron Imaging written by and published by . This book was released on 2010 with total page 34 pages. Available in PDF, EPUB and Kindle. Book excerpt: The dynamics of electronically excited helium nanodroplets are studied by femtosecond time-resolved photoelectron imaging. EUV excitation into a broad absorption band centered around 23.8 eV leads to an indirect photoemission process that generates ultraslow photoelectrons. A 1.58 eV probe pulse transiently depletes the indirect photoemission signal for pump-probe time delays

Download or read book Ultrafast dynamics in helium nanodroplets probed by XUV spectroscopy and x ray imaging written by Camila Bacellar C Silveira and published by . This book was released on 2005 with total page 107 pages. Available in PDF, EPUB and Kindle. Book excerpt: Helium nanodroplets are the smallest known objects exhibiting superfluidity, and they provide a unique cryogenic matrix for high-resolution spectroscopy and ultracold chemistry applications. The relatively simple electronic structure of helium atoms and the homogeneity of the quantum fluid clusters make them excellent model systems for the study of electronic structures and dynamics in complex systems and the emergence of collective phenomena. Coupled electronic-nuclear dynamics in laser-excited helium nanodroplets are studied in the time-domain in two distinctly different excitation regimes following either single XUV-photon excitation or strong-field ionization by a near-infrared (NIR) laser pulse. Femtosecond time- resolved XUV photoelectron spectroscopy and femtosecond time-resolved X-ray coherent diffractive imaging are employed to monitor electronic relaxation dynamics in neutral droplets and the emergence and evolution of a nanoplasma in strong-field ionized droplets, respectively. Electronically excited pure and doped He droplets are prepared using femtosecond XUV pump pulses produced by high-order harmonic generation. The excited states and subsequent relaxation dynamics are probed by ionization of transient species with a femtosecond UV probe- pulse. Pump-probe time delay-dependent photoelectron kinetic energy distributions are measured using velocity map imaging. In pure droplets excited with 23.7 eV, three dynamic pathways are identified: interband relaxation from the initially excited 1s3p,1s4p manifold to the 1s2p band, further relaxation within the 1s2p Rydberg band and rapid atomic reconfiguration involving formation of Rydberg-excited (Hen)* cores within the droplet. Ongoing efforts towards understanding energy- and charge-transfer mechanisms between the host droplets and dopant atoms are discussed. New high-harmonic generation schemes were implemented in order to directly access the lower 1s2p droplet resonances. Droplets doped with a small amounts of Kr and Ne atoms (ndopant/ndroplet

Download or read book Probing Ultrafast Electron Dynamics in Helium Nanodroplets with Deep Learning Assisted Diffraction Imaging written by Julian Claudius Zimmermann and published by . This book was released on 2021 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Synchrotron Light Sources and Free Electron Lasers written by Eberhard J. Jaeschke and published by Springer. This book was released on 2016-05-27 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: Hardly any other discovery of the nineteenth century did have such an impact on science and technology as Wilhelm Conrad Röntgen’s seminal find of the X-rays. X-ray tubes soon made their way as excellent instruments for numerous applications in medicine, biology, materials science and testing, chemistry and public security. Developing new radiation sources with higher brilliance and much extended spectral range resulted in stunning developments like the electron synchrotron and electron storage ring and the freeelectron laser. This handbook highlights these developments in fifty chapters. The reader is given not only an inside view of exciting science areas but also of design concepts for the most advanced light sources. The theory of synchrotron radiation and of the freeelectron laser, design examples and the technology basis are presented. The handbook presents advanced concepts like seeding and harmonic generation, the booming field of Terahertz radiation sources and upcoming brilliant light sources driven by laser-plasma accelerators. The applications of the most advanced light sources and the advent of nanobeams and fully coherent x-rays allow experiments from which scientists in the past could not even dream. Examples are the diffraction with nanometer resolution, imaging with a full 3D reconstruction of the object from a diffraction pattern, measuring the disorder in liquids with high spatial and temporal resolution. The 20th century was dedicated to the development and improvement of synchrotron light sources with an ever ongoing increase of brilliance. With ultrahigh brilliance sources, the 21st century will be the century of x-ray lasers and their applications. Thus, we are already close to the dream of condensed matter and biophysics: imaging single (macro)molecules and measuring their dynamics on the femtosecond timescale to produce movies with atomic resolution.

Download or read book Progress in Ultrafast Intense Laser Science XIII written by Kaoru Yamanouchi and published by Springer. This book was released on 2017-12-22 with total page 234 pages. Available in PDF, EPUB and Kindle. Book excerpt: This thirteenth volume in the PUILS series covers a broad range of topics from this interdisciplinary research field, focusing on atoms, molecules, and clusters interacting in intense laser field and high-order harmonics generation and their applications. The series delivers up-to-date reviews of progress in ultrafast intense laser science, the interdisciplinary research field spanning atomic and molecular physics, molecular science, and optical science, which has been stimulated by the developments in ultrafast laser technologies. Each volume compiles peer-reviewed articles authored by researchers at the forefront of each their own subfields of UILS. Typically, each chapter opens with an overview of the topics to be discussed, so that researchers unfamiliar to the subfield, as well as graduate students, can grasp the importance and attractions of the research topic at hand; these are followed by reports of cutting-edge discoveries.

Download or read book Nanodroplets written by Zhiming M. Wang and published by Springer Science & Business Media. This book was released on 2014-01-08 with total page 392 pages. Available in PDF, EPUB and Kindle. Book excerpt: Nanodroplets, the basis of complex and advanced nanostructures such as quantum rings, quantum dots and quantum dot clusters for future electronic and optoelectronic materials and devices, have attracted the interdisciplinary interest of chemists, physicists and engineers. This book combines experimental and theoretical analyses of nanosized droplets which reveal many attractive properties. Coverage includes nanodroplet synthesis, structure, unique behaviors and their nanofabrication, including chapters on focused ion beam, atomic force microscopy, molecular beam epitaxy and the "vapor-liquid- solid" route. Particular emphasis is given to the behavior of metallic nanodroplets, water nanodroplets and nanodroplets in polymer and metamaterial nanocomposites. The contributions of leading scientists and their research groups will provide readers with deeper insight into the chemical and physical mechanisms, properties, and potential applications of various nanodroplets.

Download or read book Unimolecular Reaction Dynamics written by Tomas Baer and published by Oxford University Press. This book was released on 1996-06-27 with total page 447 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book provides a penetrating and comprehensive description of energy selected reactions from a theoretical as well as experimental view. Three major aspects of unimolecular reactions involving the preparation of the reactants in selected energy states, the rate of dissociation of the activated molecule, and the partitioning of the excess energy among the final products, are fully discussed with the aid of 175 illustrations and over 1,000 references, most from the recent literature. Examples of both neutral and ionic reactions are presented. Many of the difficult topics are discussed at several levels of sophistication to allow access by novices as well as experts. Among the topics covered for the first time in monograph form is a discussion of highly excited vibrational/rotational states and intramolecular vibrational energy redistribution. Problems associated with the application of RRKM theory are discussed with the aid of experimental examples. Detailed comparisons are also made between different statistical models of unimolecular decomposition. Both quantum and classical models not based on statistical assumptions are described. Finally, a chapter devoted to the theory of product energy distribution includes the application of phase space theory to the dissociation of small and large clusters. The work will be welcomed as a valuable resource by practicing researchers and graduate students in physical chemistry, and those involved in the study of chemical reaction dynamics.

Download or read book Extreme States of Matter written by Vladimir E. Fortov and published by Springer. This book was released on 2015-12-26 with total page 714 pages. Available in PDF, EPUB and Kindle. Book excerpt: With its many beautiful colour pictures, this book gives fascinating insights into the unusual forms and behaviour of matter under extremely high pressures and temperatures. These extreme states are generated, among other things, by strong shock, detonation and electric explosion waves, dense laser beams, electron and ion beams, hypersonic entry of spacecraft into dense atmospheres of planets and in many other situations characterized by extremely high pressures and temperatures. Written by one of the world's foremost experts on the topic, this book will inform and fascinate all scientists dealing with materials properties and physics and also serve as an excellent introduction to plasma-, shock-wave and high-energy-density physics for students and newcomers seeking an overview. This second edition is thoroughly revised and expanded, in particular with new material on high energy-density physics, nuclear explosions and other nuclear transformation processes.

Download or read book Photoelectrocatalysis written by Leonardo Palmisano and published by Elsevier. This book was released on 2022-10-21 with total page 488 pages. Available in PDF, EPUB and Kindle. Book excerpt: Photoelectrocatalysis: Fundamentals and Applications presents an in-depth review of the topic for students and researchersworking on photoelectrocatalysis-related subjects from pure chemistry to materials and environmental chemistry inorder to propose applications and new perspectives. The main advantage of a photoelectrocatalytic process is the mildexperimental conditions under which the reactions are carried out, which are often possible at atmospheric pressure androom temperature using cheap and nontoxic solvents (e.g., water), oxidants (e.g., O2 from the air), catalytic materials (e.g.,TiO2 on Ti layer), and the potential exploitation of solar light. This book presents the fundamentals and the applications of photoelectrocatalysis, such as hydrogen production fromwater splitting, the remediation of harmful compounds, and CO2 reduction. Photoelectrocatalytic reactors and lightsources, in addition to kinetic aspects, are presented along with an exploration of the relationship between photocatalysisand electrocatalysis. In addition, photocorrosion issues and the application of selective photoelectrocatalytic organictransformations, which is now a growing field of research, are also reported. Finally, the advantages/disadvantages andfuture perspectives of photoelectrocatalysis are highlighted through the possibility of working at a pilot/industrial scale inenvironmentally friendly conditions. Presents the fundamentals of photoelectrocatalysis Outlines photoelectrocatalytic green chemistry Reviews photoelectrocatalytic remediation of harmful compounds, hydrogen production, and CO2 reduction Includes photocorrosion, photoelectrocatalytic reactors, and modeling along with kinetic aspects

Download or read book Laser Precision Microfabrication written by Koji Sugioka and published by Springer. This book was released on 2010-08-13 with total page 353 pages. Available in PDF, EPUB and Kindle. Book excerpt: Miniaturization and high precision are rapidly becoming a requirement for many industrial processes and products. As a result, there is greater interest in the use of laser microfabrication technology to achieve these goals. This book composed of 16 chapters covers all the topics of laser precision processing from fundamental aspects to industrial applications to both inorganic and biological materials. It reviews the sate of the art of research and technological development in the area of laser processing.

Download or read book Excess Electrons in Dielectric Media written by Christiane Ferradini and published by CRC Press. This book was released on 1991-08-05 with total page 454 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book provides a comprehensive review of the present knowledge and current problems concerning physical-chemical aspects of the behavior of excess electrons in various media. The book's 13 chapters strike a balance between theoretical and experimental accounts and provide in-depth presentations of specific subjects. Among the several topics discussed in this stimulating volume are primary interactions, transport, and relaxation of excess electrons of a few tens of electron-Volts in various solid and liquid materials; energetics and transport properties of electrons after thermalization in non-polar dielectric liquids; quantum simulation methods; and electron solvation in polar liquids and of excess electrons trapped in polar matrices at low temperature. Applications of these concepts are discussed as well, including hot electron transport in silicon dioxide, the fate of excess electrons created in polar dielectric liquids by photoelectrochemical methods or by cathodic generation, and excess electron production and decay in organic microheterogeneous systems. Researchers, instructors, and engineers working in the radiation sciences, condensed-matter physics, chemical physics, biophysics, photochemistry, and the biochemistry of electron transfer and electrochemistry should consider this book to be an invaluable reference resource.

Download or read book Band Ferromagnetism written by K. Baberschke and published by Springer Science & Business Media. This book was released on 2001-08-28 with total page 390 pages. Available in PDF, EPUB and Kindle. Book excerpt: The fascinating phenomenon ferromagnetism is far from being fully understood, although it surely belongs to the oldest problems of solid state physics. For any investigation it appears recommendable to distinguish between materials whose spontaneous magnetization stems from localized electrons of a partially ?lled atomic shell and those in which it is due to itinerant electrons of a partially ?lled conduction band. In the latter case one speaks of band-ferromagnetism, prototypes of which are the classical ferromagnets Fe, Co, and Ni. The present book is a status report on the remarkable progress that has recently been made towards a microscopic understanding of band-ferromagnetism as an electron c- relation e?ect. The authors of the various chapters of this book “Band-Ferromagnetism: Ground-State and Finite-Temperature Phenomena” participated as selected - perts in the 242nd WE-Heraeus-Seminar (4-6 October 2000) held under almost the same title in Wandlitz near Berlin (Germany). It was the second seminar of this type in Wandlitz. (The ?rst in 1998 dealt with the complementary topic of the physics of local-moment ferromagnets such as Gd). Twenty-six invited spe- ers from ten di?erent countries together with ?fty-?ve further participants, who presented contributions in form of posters, spent three days together discussing in an enthusiastic and fertile manner the hot topics of band-ferromagnetism.

Download or read book Astromag written by and published by . This book was released on 1988 with total page 28 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Fundamentals and Applications in Aerosol Spectroscopy written by Ruth Signorell and published by CRC Press. This book was released on 2010-12-20 with total page 513 pages. Available in PDF, EPUB and Kindle. Book excerpt: Helping you better understand the processes, instruments, and methods of aerosol spectroscopy, Fundamentals and Applications in Aerosol Spectroscopy provides an overview of the state of the art in this rapidly developing field. It covers fundamental aspects of aerosol spectroscopy, applications to atmospherically and astronomically relevant problem

Download or read book Physics and Chemistry of Finite Systems From Clusters to Crystals written by Peru Jena and published by Springer Science & Business Media. This book was released on 2013-11-11 with total page 1414 pages. Available in PDF, EPUB and Kindle. Book excerpt: Recent innovations in experimental techniques such as molecular and cluster beam epitaxy, supersonic jet expansion, matrix isolation and chemical synthesis are increasingly enabling researchers to produce materials by design and with atomic dimension. These materials constrained by sire, shape, and symmetry range from clusters containing as few as two atoms to nanoscale materials consisting of thousands of atoms. They possess unique structuraI, electronic, magnetic and optical properties that depend strongly on their size and geometry. The availability of these materials raises many fundamental questions as weIl as technological possibilities. From the academic viewpoint, the most pertinent question concerns the evolution of the atomic and electronic structure of the system as it grows from micro clusters to crystals. At what stage, for example, does the cluster look as if it is a fragment of the corresponding crystal. How do electrons forming bonds in micro-clusters transform to bands in solids? How do the size dependent properties change from discrete quantum conditions, as in clusters, to boundary constrained bulk conditions, as in nanoscale materials, to bulk conditions insensitive to boundaries? How do the criteria of classification have to be changed as one goes from one size domain to another? Potential for high technological applications also seem to be endless. Clusters of otherwise non-magnetic materials exhibit magnetic behavior when constrained by size, shape, and dimension. NanoscaIe metal particles exhibit non-linear opticaI properties and increased mechanical strength. SimiIarly, materials made from nanoscale ceramic particIes possess plastic behavior.

Download or read book Surface Science Techniques written by Gianangelo Bracco and published by Springer Science & Business Media. This book was released on 2013-01-11 with total page 668 pages. Available in PDF, EPUB and Kindle. Book excerpt: The book describes the experimental techniques employed to study surfaces and interfaces. The emphasis is on the experimental method. Therefore all chapters start with an introduction of the scientific problem, the theory necessary to understand how the technique works and how to understand the results. Descriptions of real experimental setups, experimental results at different systems are given to show both the strength and the limits of the technique. In a final part the new developments and possible extensions of the techniques are presented. The included techniques provide microscopic as well as macroscopic information. They cover most of the techniques used in surface science.

Download or read book Analytical Chemistry for Cultural Heritage written by Rocco Mazzeo and published by Springer. This book was released on 2017-01-25 with total page 370 pages. Available in PDF, EPUB and Kindle. Book excerpt: The series Topics in Current Chemistry Collections presents critical reviews from the journal Topics in Current Chemistry organized in topical volumes. The scope of coverage is all areas of chemical science including the interfaces with related disciplines such as biology, medicine and materials science. The goal of each thematic volume is to give the non-specialist reader, whether in academia or industry, a comprehensive insight into an area where new research is emerging which is of interest to a larger scientific audience.Each review within the volume critically surveys one aspect of that topic and places it within the context of the volume as a whole. The most significant developments of the last 5 to 10 years are presented using selected examples to illustrate the principles discussed. The coverage is not intended to be an exhaustive summary of the field or include large quantities of data, but should rather be conceptual, concentrating on the methodological thinking that will allow the non-specialist reader to understand the information presented. Contributions also offer an outlook on potential future developments in the field.