Download or read book Spectroscopic Applications of Terahertz Quantum Cascade Lasers written by Tasmim Alam and published by Cuvillier Verlag. This book was released on 2020-10-29 with total page 132 pages. Available in PDF, EPUB and Kindle. Book excerpt: Quantum cascade lasers (QCLs) are attractive for high-resolution spectroscopy because they can provide high power and a narrow linewidth. They are particularly promising in the terahertz (THz) range since they can be used as local oscillators for heterodyne detection as well as transmitters for direct detection. However, THz QCL-based technologies are still under development and are limited by the lack of frequency tunability as well as the frequency and output power stability for free-running operation. In this dissertation, frequency tuning and linewidth of THz QCLs are studied in detail by using rotational spectroscopic features of molecular species. In molecular spectroscopy, the Doppler eff ect broadens the spectral lines of molecules in the gas phase at thermal equilibrium. Saturated absorption spectroscopy has been performed that allows for sub-Doppler resolution of the spectral features. One possible application is QCL frequency stabilization based on the Lamb dip. Since the tunability of the emission frequency is an essential requirement to use THz QCL for high-resolution spectroscopy, a new method has been developed that relies on near-infrared (NIR) optical excitation of the QCL rear-facet. A wide tuning range has been achieved by using this approach. The scheme is straightforward to implement, and the approach can be readily applied to a large class of THz QCLs. The frequency and output stability of the local oscillator has a direct impact on the performance and consistency of the heterodyne spectroscopy. A technique has been developed for a simultaneous stabilization of the frequency and output power by taking advantage of the frequency and power regulation by NIR excitation. The results presented in this thesis will enable the routine use of THz QCLs for spectroscopic applications in the near future.

Download or read book Terahertz Quantum cascade Lasers for Spectroscopic Applications written by Benjamin Malte Röben and published by . This book was released on 2018 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Novel Applications of Terahertz Quantum Cascade Lasers written by Binbin Wei and published by . This book was released on 2020 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Mid Infrared and Terahertz Quantum Cascade Lasers written by Dan Botez and published by Cambridge University Press. This book was released on 2023-09-14 with total page 552 pages. Available in PDF, EPUB and Kindle. Book excerpt: Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.

Download or read book Mid Infrared and Terahertz Quantum Cascade Lasers written by Dan Botez and published by Cambridge University Press. This book was released on 2023-06-30 with total page 551 pages. Available in PDF, EPUB and Kindle. Book excerpt: A state-of-the-art overview of this rapidly expanding field, featuring fundamental theory, practical applications, and real-life examples.

Download or read book Quantum Cascade Lasers for Terahertz Applications written by Sudeep Khanal and published by . This book was released on 2017 with total page 241 pages. Available in PDF, EPUB and Kindle. Book excerpt: The mid-infrared (lambda ~ 3 -- 30 mum) and terahertz (THz) or far-infrared (lambda ~ 30 -- 300 mum) regions of the electromagnetic spectrum offer unique applications in spectroscopy, sensing, and imaging. However, these longer wavelengths (photon energies 0.4 eV) are difficult to generate with compact solid-state devices owing to the lack of naturally occurring materials with small bandgaps. Quantum-cascade lasers (QCLs) are unipolar devices based on semiconductor superlattices, in which radiation occurs due to intersubband (rather than interband) optical transitions.

Download or read book Physics and Applications of Terahertz Radiation written by Matteo Perenzoni and published by Springer. This book was released on 2013-10-16 with total page 257 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book covers the latest advances in the techniques employed to manage the THz radiation and its potential uses. It has been subdivided in three sections: THz Detectors, THz Sources, Systems and Applications. These three sections will allow the reader to be introduced in a logical way to the physics problems of sensing and generation of the terahertz radiation, the implementation of these devices into systems including other components and finally the exploitation of the equipment for real applications in some different field. All of the sections and chapters can be individually addressed in order to deepen the understanding of a single topic without the need to read the whole book. The THz Detectors section will address the latest developments in detection devices based on three different physical principles: photodetection, thermal power detection, rectification. The THz Sources section will describe three completely different generation methods, operating in three separate scales: quantum cascade lasers, free electron lasers and non-linear optical generation. The Systems and Applications section will take care of introducing many of the aspects needed to move from a device to an equipment perspective: control of terahertz radiation, its use in imaging or in spectroscopy, potential uses in security, and will address also safety issues. The text book is at a level appropriate to graduate level courses up to researchers in the field who require a reference book covering all aspects of terahertz technology.

Download or read book Development of Terahertz QCLs written by Sushil Kumar (Ph. D.) and published by . This book was released on 2007 with total page 340 pages. Available in PDF, EPUB and Kindle. Book excerpt: The terahertz or the far-infrared frequency range of the electromagnetic spectrum (...) has historically been technologically underdeveloped despite having many potential applications, primarily due to lack of suitable sources of coherent radiation. Following on the remarkable development of mid-infrared (...) quantum-cascade lasers (QCLs) in the past decade, this thesis describes the development of electrically-pumped terahertz quantum-cascade lasers in GaAs/AlsGal_. As heterostructures that span a spectral range of 1.59 - 5.0 THz (...). A quantum-cascade laser (QCL) emits photons due to electronic intersubband transitions in the quantum-wells of a semiconductor heterostructure. The operation of terahertz QCLs at frequencies below the Reststrahlen band in the semiconductor (...), is significantly more challenging as compared to that of the mid-infrared QCLs. Firstly, due to small energy separation between the laser levels various intersubband scattering mechanisms are activated, which make it difficult to selectively depopulate the lower laser level. Additionally, as electrons gain enough kinetic energy in the upper laser level thermally activated longitudinal-optical (LO) phonon scattering reduces the level lifetime and makes it difficult to sustain population inversion at higher temperatures. Secondly, waveguide design for terahertz mode confinement is also more challenging due to higher free-carrier losses in the semiconducting doped regions at the terahertz frequencies. For successful designs reported in this work, the lower radiative state depopulation is achieved by a combination of resonant-tunneling and fast LO phonon scattering, which allow robust operation even at relatively high temperatures. An equally important enabling mechanism for these lasers is the development of metal-metal waveguides, which provide low waveguides losses, and strong mode confinement due to subwavelength mode localization in the vertical dimension. With these techniques some record performances for terahertz QCLs are demonstrated including the highest pulsed operating temperature of 169 K, the highest continuous-wave (cw) operating temperature of 117 K, and the highest optical power output (248 mW in pulsed and 138 mW in cw at 5 K) for any terahertz QCL. Towards the bigger goal of realizing a 1-THz solid-state laser to ultimately bridge the gap between electronic and optical sources of electromagnetic radiation, QCLs with a unique one-well injection scheme, which minimizes intersubband absorption losses that occur at longer wavelengths, are developed. Based on this scheme a QCL operating at 1.59 THz (A - 189 ym) is realized, which is amongst the lowest frequency solid-state lasers that operate without the assistance of a magnetic field. This thesis also reports on the development of distributed-feedback lasers in metal-metal waveguides to obtain single-mode operation, with greater output power and better beam quality. The subwavelength vertical dimension in these waveguides leads to a strongly coupled DFB action and a large reflection from the end-facets, and thus conventional coupled-mode theory is not directly applicable to the DFB design. A design technique with precise control of phase of reflection at the end-facets is developed with the aid of finite-element analysis, and with some additional unique design and fabrication methods, robust DFB operation has been obtained. Single-mode surface-emitting terahertz QCLs operating up to - 150 K are demonstrated, with different grating devices spanning a range of approximately 0.35 THz around v - 3 THz using the same gain medium. A single-lobed far-field radiation pattern, higher output power due to surface-emission, and a relatively small degradation in temperature performance compared to the Fabry-Perot ridge lasers makes these DFB lasers well suited for practical applications that are being targeted by the terahertz quantum-cascade lasers.

Download or read book Terahertz Quantum Cascade Lasers for Astronomical Applications written by Dana Turcinkova and published by . This book was released on 2014 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Ultra fast Spectroscopy of Terahertz Quantum Cascade Lasers written by Sergej Markmann and published by . This book was released on 2016 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Widely Tunable Terahertz Semiconductor Laser Sources written by Aiting Jiang and published by . This book was released on 2015 with total page 204 pages. Available in PDF, EPUB and Kindle. Book excerpt: Terahertz Quantum Cascade Lasers (THz QCLs) and Terahertz Difference Frequency Generation Quantum Cascade Laser sources (DFG-QCLs) are two types of semiconductor THz radiation sources that are compact and amenable to production in mass quantities. THz QCL can generate over 1W of power under cryogenic temperatures, while THz DFG-QCL can be operated under room temperature over 1mW level output. For either case, widely tunable solution is highly desired for spectroscopy applications. For THz QCLs, operation is still limited to cryogenic temperature and broad tuning is not available. Our experimental study shows that using variable barriers is a viable approach to enhance the design space for THz QCLs. We also propose to tune the spectral output of these devices using an optically projected variable distributed feedback grating. Tuning will be achieved by changing the projected grating period. Preliminary experimental results support the idea but higher pumping light intensity is required for this method to work. For THz DFG-QCLs, very broad tuning in 1-6 THz range has been demonstrated using rotating diffraction grating in an external cavity setup. Similar tuning range can also be achieved in a monolithic configuration. Based on the previous work which demonstrated an electrical monolithic tuner with 580 GHz tuning range, we design and test in this dissertation a linear array of 10 DFG-QCL devices to cover a 2 THz tuning range. An independent gain control scheme is developed to achieve high yield (~100%) of individual device. It is implemented via independent current pumping of two electrically isolated sections. Surface DFB grating and independent current pumping scheme used in our DFG QCLs is found to be useful for mid-IR QCL array sources. We propose a longitudinal integration scheme of multiple grating sections. It enables a single ridge to emit single mode radiation at different wavelengths upon selection. This helps to reduce mid-IR QCL array far field span. We demonstrated single ridge devices that can emit 2 or 3 different wavelengths upon selection.

Download or read book The Development and Applications of Terahertz Quantum Cascade Lasers written by Raed Hussain S. Alhathlool and published by . This book was released on 2014 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Download or read book Magneto spectroscopy and Development of Terahertz Quantum Cascade Lasers written by and published by . This book was released on with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: In this work we concentrate our efforts on the generation of laser emission at low THz frequencies (3-1 THz range) employing the quantum cascade technology. Quantum cascade (QC) lasers are unipolar semiconductor lasers based on intersubband transitions in quantum wells that cover a large portion of the Mid and Far Infrared electromagnetic spectrum. Two main research lines have been followed: (i) the development of quantum cascade lasers based on population inversion between parabolic subbands and (ii) the development of low frequency QC lasers based on a three-dimensional electron confinement induced by an external magnetic field. (i) : Gain and laser action have been demonstrated in different systems at frequencies of 3.4 3.6 THz exploiting bound-to-bound and bound-to-continuum optical transition. A QC laser emitting at 3.6 THz and based on a vertical transition and resonant tunneling in a single quantum well has been demonstrated. To overcome the limitations in performance of such a system, an heterostructure laser based on a bound-to-continuum transition has been developed. The structure was the first one to operate above the technologically important temperature of liquid nitrogen. With a further development of the bound-to-continuum design that includes lower state lifetime reduction by optical phonon emission, laser action was successfully achieved at 115 K.A study of different waveguide mechanisms suitable for different THz frequencies has also been carried out. (ii) : THz quantum cascade lasers based on the in-plane confinement introduced by a strong magnetic field applied perpendiculary to the plane of the layers have been developed. A model system based on large single quantum wells (50-60 nm wide) has been exploited to study this gain mechanism. Such an approach led to the extension of the frequency range of operation of QC lasers, with the demonstration of laser action at 1.39 THz (220 mm) which is the lowest frequency observed to-date for this kind of.

Download or read book Modern Techniques of Spectroscopy written by Dheeraj Kumar Singh and published by Springer Nature. This book was released on 2021-04-01 with total page 663 pages. Available in PDF, EPUB and Kindle. Book excerpt: The book highlights recent developments in the field of spectroscopy by providing the readers with an updated and high-level of overview. The focus of this book is on the introduction to concepts of modern spectroscopic techniques, recent technological innovations in this field, and current examples of applications to molecules and materials relevant for academia and industry. The book will be beneficial to researchers from various branches of science and technology, and is intended to point them to modern techniques, which might be useful for their specific problems. Spectroscopic techniques, that are discussed include, UV-Visible absorption spectroscopy, XPS, Raman spectroscopy, SERS, TERS, CARS, IR absorption spectroscopy, SFG, LIBS, Quantum cascade laser (QCL) spectroscopy, fluorescence spectroscopy, ellipsometry, cavity-enhanced absorption spectroscopy, such as cavity ring-down spectroscopy (CRDS) and evanescent wave-CRDS both in gas and condensed phases, time-resolved spectroscopy etc. Applications introduced in the different chapters demonstrates the usefulness of the spectroscopic techniques for the characterization of fundamental properties of molecules, e.g. in connection with environmental impact, bio-activity, or usefulness for pharmaceutical drugs, and materials important e.g. for nano-science, nuclear chemistry, or bio-applications. The book presents how spectroscopic techniques can help to better understand substances, which have also great impact on questions of social and economic relevance (environment, alternative energy, etc.).

Download or read book Towards Terahertz Dual comb Spectroscopy Based on Quantum Cascade Lasers written by and published by . This book was released on 2015 with total page 99 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this thesis, terahertz (THz) laser frequency combs are improved and THz dual-comb spectroscopy method is demonstrated. To achieve better performance of THz quantum cascade laser (QCL) frequency combs, several broadband homogeneous and heterogeneous gain media are characterized, and corresponding dispersion compensators are designed. All THz QCL frequency combs are fabricated in Microsystems Technology Laboratories at MIT using our group's standard process. By utilizing the broad spectral coverage of THz QCL frequency combs and the multiheterodyne detection method, a prototype of the THz dual-comb spectrometer is demonstrated. This thesis work provides an important step towards realizing laser-based broadband THz spectroscopy system for chemical identification and explosive detection.

Download or read book Terahertz and Mid Infrared Radiation written by Mauro Pereira and published by Springer Science & Business Media. This book was released on 2011-02-26 with total page 218 pages. Available in PDF, EPUB and Kindle. Book excerpt: Terahertz (THz) and Mid-Infrared (MIR) radiation (TERA-MIR) can be transmitted through nearly any material without causing biological harm. Novel and rapid methods of detection can be created with devices operation in these spectral ranges allowing scanning for weapons, detecting hidden explosives (including plastic landmines), controlling the quality of food and a host of other exciting applications. This book focuses on mathematical and physical aspects of the field, on unifying these two spectral domains (THz and MIR) with regard to common sources, detectors, materials and applications, and on key interdisciplinary topics. The main THz and MIR source is the quantum cascade laser (QCL). Thus significant attention is paid to the challenge of turning this advanced technology into affordable commercial devices so as to exploit its enormous potential. However other alternatives to THz QCLs are also presented, e.g. sub-terahertz imaging from avalanching GaAs bipolar transistors, Josephson junctions as THz sources, semiconductor materials for pulsed THz sources, superconducting THz electronics with Josephson vortices. In summary this book delivers a global picture of the state of the art in TERA-MIR generation, detection and applications.

Download or read book Optimization of a Quantum Cascade Laser Operating in the Terahertz Frequency Range Using a Multiobjective Evolutionary Algorithm written by Traci A. Keller and published by . This book was released on 2004-06-01 with total page 125 pages. Available in PDF, EPUB and Kindle. Book excerpt: A quantum cascade (QC) laser is a specific type of semiconductor laser that operates through principles of quantum mechanics. In less than a decade QC lasers are already able to outperform previously designed double heterostructure semiconductor lasers. Because there is a genuine lack of compact and coherent devices which can operate in the far-infrared region the motivation exists for designing a terahertz QC laser. A device operating at this frequency is expected to be more efficient and cost effective than currently existing devices. It has potential applications in the fields of spectroscopy, astronomy, medicine and free-space communication as well as applications to near-space radar and chemical/biological detection. The overarching goal of this research was to find QC laser parameter combinations which can be used to fabricate viable structures. To ensure operation in the THz region the device must conform to the extremely small energy level spacing range from Æ10-15 meV. The time and expense of the design and production process is prohibitive, so an alternative to fabrication was necessary. To accomplish this goal a model of a QC laser, developed at Worchester Polytechnic Institute with sponsorship from the Air Force Research Laboratory Sensors Directorate, and the General Multiobjective Parallel Genetic Algorithm (GenMOP), developed at the Air Force Institute of Technology, were integrated to form a computer simulation which stochastically searches for feasible solutions.