Download or read book Inner shell Photoemission from Atoms and Molecules Using Synchrotron Radiation written by Dennis William Lindle and published by . This book was released on 1983 with total page 276 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Inner shell Photoemission from Atoms and Molecules Using Synchrotron Radiation written by and published by . This book was released on 1983 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Photoelectron spectroscopy, in conjunction with synchrotron radiation, has been used to study inner-shell photoemission from atoms and molecules. The time structure of the synchrotron radiation permits the measurements of time-of-flight (TOF) spectra of Auger and photoelectrons, thereby increasing the electron collection efficiency. The double-angle TOF method yielded angle-resolved photoelectron intensities, which were used to determine photoionization cross sections and photoelectron angular distributions in several cases. Comparison to theoretical calculations has been made where possible to help explain observed phenomena in terms of the electronic structure and photoionization dynamics of the systems studied. 154 references, 23 figures, 7 tables.
Download or read book Electron Spectrometry of Atoms Using Synchrotron Radiation written by Volker Schmidt and published by Cambridge University Press. This book was released on 1997-05-15 with total page 454 pages. Available in PDF, EPUB and Kindle. Book excerpt: The study of electron spectrometry using synchrotron radiation is a growing field of research driven by the increasing availability of advanced synchrotron radiation light sources and improved theoretical methods for solving the many-electron problem in atoms. This balanced account, by a leading researcher in this field, will be of value to both theorists and experimentalists in atomic, molecular and chemical physicists.
Download or read book Inner Shell and X Ray Physics of Atoms and Solids written by Derek Fabian and published by Springer Science & Business Media. This book was released on 2013-04-18 with total page 947 pages. Available in PDF, EPUB and Kindle. Book excerpt: A wide range of atomic and solid state phenomena is studied today by means of x-ray excitation or inner-shell ionization, as this volume strikingly illustrates. The strong link between these two fields of investigation is partly the result of the extensive developments within each and also largely due to the broad variety of theoretical and experimental techniques now available. All im portant recent advances are to be found highlighted here; most are substantially reviewed. Two dominant research threads are evident in, the chapters of this book. While clearly distinguishable, they are inescapably en twined. One is concerned with x-ray processes as probes for the study of solid-state effects, the other with the measurement and interpretation of inner-shell and bremsstrahlung processes in iso lated systems. In the first, a given material is made the target in an x-ray tube; in the second, free atoms form the target while a solid material can be used when the effect of the solid environ ment on the excitation processes is negligible. Thus, although inner-shell ionization is predominantly concerned with atoms and x-ray processes with the solid state, there are large regions of overlap which have arisen when a given research technique has de veloped from studies in both areas. To bring out these features we have arranged the chapters in the order: atomic, solid-state, chemical.
Download or read book Atomic and Molecular Photoelectron and Auger Electron SpectroscopyStudies Using Synchrotron Radiation written by and published by . This book was released on 1982 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Electron spectroscopy, combined with synchrotron radiation, was used to measure the angular distributions of photoelectrons and Auger electrons from atoms and molecules as functions of photon energy. The branching ratios and partial cross sections were a 130 measured in certain cases. By comparison with theoretical calculations, the experimental results are interpreted in terms of the characteristic electronic structure and ionization dynamics of the atomic or molecular sample. The time structure of the synchrotron radiation source was used to record time-of-flight (TOF) spectra o f the ejected electrons. The ''a double-angle-TOF'' method for the measurement of photoelectron angular distributions is discussed. This technique offers the advantages of increased electron collect ion efficiency and the elimination of certain systematic errors. Several results were obtained for Xe using photon energies in the range hv C"60-190 eV, where excitation and ionization of the inner-subshell 4d electrons dominates. The 4d asymmetry parameter? exhibits strong oscillations with energy, in agreement with several theoretical calculations. As predicted, the 5p asymmetry parameter was observed to deviate strongly from that calculated using the independent-electron model, due to intershell correlation with the 4d electrons.
Download or read book Atomic Inner Shell Physics written by Bernd Crasemann and published by Springer Science & Business Media. This book was released on 2013-03-09 with total page 760 pages. Available in PDF, EPUB and Kindle. Book excerpt: The physics of atomic inner shells has undergone significant advances in recent years. Fast computers and new experimental tools, notably syn chrotron-radiation sources and heavy-ion accelerators, have greatly enhan ced the scope of problems that are accessible. The level of research activity is growing substantially; added incentives are provided by the importance of inner-shell processes in such diverse areas as plasma studies, astrophysics, laser technology, biology, medicine, and materials science. The main reason for all this exciting activity in atomic inner-shell physics, to be sure, lies in the significance of the fundamental problems that are coming within grasp. The large energies of many inner-shell processes cause relativistic and quantum-electrodynamic effects to become strong. Unique opportunities exist for delicate tests of such phenomena as the screening of the electron self-energy and the limits of validity of the present form of the frequency-dependent Breit interaction, to name but two. The many-body problem, which pervades virtually all of physics, presents somewhat less intractable aspects in the atomic inner-shell regime: correlations are relatively weak so that they can be treated perturbatively, and the basic potential is simple and known! The dynamics of inner-shell processes are characterized by exceedingly short lifetimes and high transition rates that strain perturbation theory to its limits and obliterate the traditional separation of excitation and deexcitation. These factors are only now being explored, as are interference phenomena between the various channels.
Download or read book Photoabsorption Photoionization and Photoelectron Spectroscopy written by Joseph Berkowitz and published by Academic Press. This book was released on 2012-12-02 with total page 490 pages. Available in PDF, EPUB and Kindle. Book excerpt: Photoabsorption, Photoionization, and Photoelectron Spectroscopy explores photoabsorption processes involving individual, isolated molecules in the wavelength or photon energy range from the ionization thresholds of molecules (usually in the vacuum ultraviolet region) through the soft and hard X-ray region and beyond the ""K edge."" The interaction between electromagnetic radiation and isolated molecules based on photoabsorption, photoionization, and photoelectron spectroscopy studies is described, along with the techniques for measurement of total and partial cross sections. This book is comprised of eight chapters and examines the decomposition of molecules and molecular ions as well as mildly excited (valence shell excitation) and highly excited (inner shell excitation) molecules. After providing a general theoretical background, it discusses certain classes of atoms and molecules and considers electromagnetic interactions with gases. The following chapters focus on photoabsorption below the first ionization limit; quasi-discrete states above the first ionization potential; and the ionization continuum. Total photoabsorption and photoionization cross sections for selected molecules are also considered, and the angular distribution of photoelectrons is analyzed. The various measurement techniques are described in the last chapter. This monograph will be of interest to radiation chemists, radiation physicists, photochemists, mass spectrometrists, and perhaps radiation biologists.
Download or read book Synchrotron Radiation Inner shell Photoionization of Atomic and Molecular Gases written by and published by . This book was released on 1986 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: A time-of-flight (TOF) spectrometer has been used to measure the average kinetic energies of near thermal atomic and molecular ions, as well as energetic molecular ion fragments, produced by inner-shell photoionization of atomic and molecular gas targets using x rays from the National Synchrotron Light Source (NSLS). While atomic and molecular ions acquire very little energy from the initial photoionization event and subsequent vacancy cascades, multiply charged molecular ions decompose rapidly, producing fragment ions which have kinetic energies determined by their configuration at the moment of decomposition. The strong effects observed suggest that this technique may be extended to the study of configurations of free molecules as well as the orientation of molecules adsorbed on surfaces. 5 refs., 2 figs.
Download or read book Controlling the Quantum World written by National Research Council and published by National Academies Press. This book was released on 2007-06-21 with total page 245 pages. Available in PDF, EPUB and Kindle. Book excerpt: As part of the Physics 2010 decadal survey project, the Department of Energy and the National Science Foundation requested that the National Research Council assess the opportunities, over roughly the next decade, in atomic, molecular, and optical (AMO) science and technology. In particular, the National Research Council was asked to cover the state of AMO science, emphasizing recent accomplishments and identifying new and compelling scientific questions. Controlling the Quantum World, discusses both the roles and challenges for AMO science in instrumentation; scientific research near absolute zero; development of extremely intense x-ray and laser sources; exploration and control of molecular processes; photonics at the nanoscale level; and development of quantum information technology. This book also offers an assessment of and recommendations about critical issues concerning maintaining U.S. leadership in AMO science and technology.
Download or read book Photoionization and Other Probes of Many Electron Interactions written by F. Wuilleumier and published by Springer Science & Business Media. This book was released on 2013-11-21 with total page 474 pages. Available in PDF, EPUB and Kindle. Book excerpt: The Advanced Study Institute on "Photoionization and Other Probes of Many-Electron Interactions" was held at the Centre "Les Cigales" in Carry-Ie-Rouet (France), from August 31st till September 13th 1975. The Institute was sponsored by the Scienti fic Affairs Division of NATO. The "Centre National de la Recher che Scientifique" (France) gave also partial support to the French participants and the National Science Foundation (U. S . A. ) to the American participants. A total of 18 lecturers, and 54 students selected among more than 120 applicants, attended the Institute. Over the last few years, substantial progress has been made in the experimental study of photon- or electron interactions with atoms. In particular, the g. rowing number of facilities created to use the synchrotron radiation makes now possible the realization of new types of experiments. The accumulation of new results showed clearly it was necessary to introduce electron correlations in the theoretical models in order to explain the existence and the probability of a large number of processes, in particular multiple processes. Thus large progress has also been made in the theore tical description of the excitation of the electronic systems and their interactions. It was the purpose of this Institute to bring together theoreticians and experimentalists in order to provide an opportunity to present in details the state of the art, in experiment as well as in theory, and to favor discussions on future experimen tal and theoretical studies.
Download or read book Photoionization of Atoms and Small Molecules Using Synchrotron Radiation SF6 SiF4 written by and published by . This book was released on 1986 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The combination of synchrotron radiation and time-of-flight electron spectroscopy has been used to study the photoionization dynamics of atoms (Li) and small molecules (SF6, SiF4, and SO2). Partial cross sections and angular distribution asymmetry parameters have been measured for Auger electrons and photoelectrons as functions of photon energy. Emphasis is on the basic understanding of electron correlation and resonant effects as manifested in the photoemission spectra for these systems. 254 refs., 46 figs., 10 tabs.
Download or read book Scientific and Technical Aerospace Reports written by and published by . This book was released on 1985 with total page 1346 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Molecular Photoemission Studies Using Synchrotron Radiation written by Carlton Maurice Truesdale and published by . This book was released on 1983 with total page 428 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Inner Shell and X Ray Physics of Atoms and Solids written by Derek J. Fabian and published by Springer. This book was released on 1981-11 with total page 988 pages. Available in PDF, EPUB and Kindle. Book excerpt: A wide range of atomic and solid state phenomena is studied today by means of x-ray excitation or inner-shell ionization, as this volume strikingly illustrates. The strong link between these two fields of investigation is partly the result of the extensive developments within each and also largely due to the broad variety of theoretical and experimental techniques now available. All im portant recent advances are to be found highlighted here; most are substantially reviewed. Two dominant research threads are evident in, the chapters of this book. While clearly distinguishable, they are inescapably en twined. One is concerned with x-ray processes as probes for the study of solid-state effects, the other with the measurement and interpretation of inner-shell and bremsstrahlung processes in iso lated systems. In the first, a given material is made the target in an x-ray tube; in the second, free atoms form the target while a solid material can be used when the effect of the solid environ ment on the excitation processes is negligible. Thus, although inner-shell ionization is predominantly concerned with atoms and x-ray processes with the solid state, there are large regions of overlap which have arisen when a given research technique has de veloped from studies in both areas. To bring out these features we have arranged the chapters in the order: atomic, solid-state, chemical.
Download or read book Chemical Applications of Synchrotron Radiation written by Tsun-Kong Sham and published by World Scientific. This book was released on 2002 with total page 663 pages. Available in PDF, EPUB and Kindle. Book excerpt: The synchrotron light source is becoming widely available, after its evolution from its infancy in the sixties to the present third generation source with insertion devices. It is timely to examine the impact that synchrotron light has made and will continue to make on chemical research. With this objective in mind, the editor of this invaluable book invited contributions from practitioners who are in the forefront of the research. The book summarizes most of the significant developments in the last decade in chemical and related research using synchrotron light. The utilization of the light as a probe as well as an energy source is emphasized.This book is organized into two parts, in order of increasing photon energy. Part I deals with the applications of low energy photons and covers areas such as gas phase photodissociation reactions and dynamics, soft X-ray fluorescence, IR and photoemission analysis of surfaces, spectroscopy of organic and polymeric materials, catalysts, electronic and magnetic materials, and spectromicroscopy. Part II encompasses applications using soft to hard X-rays, including spectroscopy of surface and thin films, XAFS, diffraction and scattering, and several technological applications, namely the microprobe, photoetching and tribology.
Download or read book Photoionization of Atoms and Small Molecules Using Synchroton Radiation written by Tricia Anne Ferrett and published by . This book was released on 1986 with total page 548 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Dynamical Processes in Atomic and Molecular Physics written by Gennadi Ogurtsov and published by Bentham Science Publishers. This book was released on 2012 with total page 128 pages. Available in PDF, EPUB and Kindle. Book excerpt: Atomic and molecular physics underlie a basis for our knowledge of fundamental processes in nature and technology and in such applications as solid state physics, chemistry and biology. In recent years, atomic and molecular physics has undergone a revolutionary change due to great achievements in computing and experimental techniques. As a result, it has become possible to obtain information both on atomic and molecular characteristics and on dynamics of atomic and molecular processes. This e-book highlights the present state of investigations in the field of atomic and molecular physics. Recent theoretical developments as well as new discoveries and observations are discussed. the Book should be of interest to students studying atomic and molecular physics and specialists in related fields of science and technology.
