Download or read book High Flux Isolated Attosecond Pulse Generation written by Yi Wu and published by . This book was released on 2013 with total page 138 pages. Available in PDF, EPUB and Kindle. Book excerpt: This thesis outlines the high intensity tabletop attosecond extreme ultraviolet laser source at the Institute for the Frontier of Attosecond Science and Technology Laboratory. First, a unique Ti:Sapphire chirped pulse amplifier laser system that delivers 14 fs pulses with 300 mJ energy at a 10 Hz repetition rate was designed and built. The broadband spectrum extending from 700 nm to 900 nm was obtained by seeding a two stage Ti:Sapphire chirped pulse power amplifier with mJ-level white light pulses from a gas filled hollow core fiber. It is the highest energy level ever achieved by a broadband pulse in a chirped pulse amplifier up to the current date. Second, using this laser as a driving laser source, the generalized double optical gating method is employed to generate isolated attosecond pulses. Detailed gate width analysis of the ellipticity dependent pulse were performed. Calculation of electron light interaction dynamics on the atomic level was carried out to demonstrate the mechanism of isolated pulse generation. Third, a complete diagnostic apparatus was built to extract and analyze the generated attosecond pulse in spectral domain. The result confirms that an extreme ultraviolet super continuum supporting 230 as isolated attosecond pulses at 35 eV was generated using the generalized double optical gating technique. The extreme ultraviolet pulse energy was 100 nJ at the exit of the argon gas target.
Download or read book Towards High flux Isolated Attosecond Pulses with a 200 TW CPA written by Eric Cunningham and published by . This book was released on 2015 with total page 194 pages. Available in PDF, EPUB and Kindle. Book excerpt: To obtain the microjoule-level attosecond pulse energy required for performing all-attosecond experiments, the attosecond flux generated by the IFAST 10 TW system was still deficient by an order of magnitude. To this end, the laser system was upgraded to provide joule-level output energies while maintaining pulse compression to 15 fs, with a targeted peak power of 200 TW. This was accomplished by adding an additional Ti:sapphire amplifier to the existing 10 TW system and implementing a new pulse compression system to accommodate the higher pulse energy. Because this system operated at a 10 Hz repetition rate, stabilization of the carrier-envelope phase (CEP)--important for controlling attosecond pulse production--could not be achieved using traditional methods. Therefore, a new scheme was developed, demonstrating the first-ever control of CEP in a chirped-pulse amplifier (CPA) at low repetition rates. Finally, a new variation of optical gating was proposed as a way to improve the efficiency of the attosecond pulse generation process. This method was also predicted to allow for the generation of isolated attosecond pulses with longer driving laser pulses, as well as the extension of the highenergy photon cut-off of the XUV continuum.
Download or read book Generation of High flux Attosecond Pulses and Towards Attosecond attosecond Pump probe Experiments written by Yang Wang and published by . This book was released on 2017 with total page 143 pages. Available in PDF, EPUB and Kindle. Book excerpt: At present, the energy of a single isolated attosecond pulse is limited to nanojoule levels. As a result, an intense femtosecond pulse has always been used in combination with a weak attosecond pulse in time-resolved experiments. To reach the goal of conducting true attosecond pump-attosecond probe experiments, a high flux laser source has been developed that can potentially deliver microjoule level isolated attosecond pulses in the 50 eV range, and a unique experimental end station has been fabricated and implemented that can provide precision control of the attosecond-attosecond pump-probe pulses. In order to scale up the attosecond flux, a unique Ti:-Sapphire laser system with a three-stage amplifier that delivers pulses with a 2 J energy at a 10 Hz repetition rate was designed and built. The broadband pulse spectrum covering from 700 nm to 900 nm was generated, supporting a pulse duration of 12 fs. The high flux high-order harmonics were generated in a gas tube filled with argon by a loosely focused geometry under a phase-matching condition. The wavefront distortions for the driving laser were corrected by a deformable mirror with a Shack-Hartmann sensor to significantly improve the extreme ultraviolet radiation conversion efficiency due to the excellent beam profile at focus. A high-damage-threshold beam splitter is demonstrated to eliminate energetic driving laser pulses from high-order harmonics. The extreme ultraviolet pulse energy is measured to be 0.3 microjoule at the exit of the argon gas target. The experimental facilities developed will lead to the generation of microjoule level isolated attosecond pulses and the demonstration of true atto pump-atto probe experiments in near future. Finally, in experiment, we show the first demonstration of carrier-envelope phase controlled filamentation in air using millijoule-level few-cycle mid-infrared laser pulses.
Download or read book Double Optical Gating written by Steve Gilbertson and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The observation and control of dynamics in atomic and molecular targets requires the use of laser pulses with duration less than the characteristic timescale of the process which is to be manipulated. For electron dynamics, this time scale is on the order of attoseconds where 1 attosecond = 10[superscript]-18 seconds. In order to generate pulses on this time scale, different gating methods have been proposed. The idea is to extract or "gate" a single pulse from an attosecond pulse train and switch off all the other pulses. While previous methods have had some success, they are very difficult to implement and so far very few labs have access to these unique light sources. The purpose of this work is to introduce a new method, called double optical gating (DOG), and to demonstrate its effectiveness at generating high contrast single isolated attosecond pulses from multi-cycle lasers. First, the method is described in detail and is investigated in the spectral domain. The resulting attosecond pulses produced are then temporally characterized through attosecond streaking. A second method of gating, called generalized double optical gating (GDOG), is also introduced. This method allows attosecond pulse generation directly from a carrier-envelope phase un-stabilized laser system for the first time. Next the methods of DOG and GDOG are implemented in attosecond applications like high flux pulses and extreme broadband spectrum generation. Finally, the attosecond pulses themselves are used in experiments. First, an attosecond/femtosecond cross correlation is used for characterization of spatial and temporal properties of femtosecond pulses. Then, an attosecond pump, femtosecond probe experiment is conducted to observe and control electron dynamics in helium for the first time.
Download or read book Generation and Characterization of Sub 70 Isolated Attosecond Pulses written by Qi Zhang and published by . This book was released on 2014 with total page 115 pages. Available in PDF, EPUB and Kindle. Book excerpt: Dynamics occurring on microscopic scales, such as electronic motion inside atoms and molecules, are governed by quantum mechanics. However, the Schrödinger equation is usually too complicated to solve analytically for systems other than the hydrogen atom. Even for some simple atoms such as helium, it still takes months to do a full numerical analysis. Therefore, practical problems are often solved only after simplification. The results are then compared with the experimental outcome in both the spectral and temporal domain. For accurate experimental comparison, temporal resolution on the attosecond scale is required. This had not been achieved until the first demonstration of the single attosecond pulse in 2001. After this breakthrough, "attophysics" immediately became a hot field in the physics and optics community. While the attosecond pulse has served as an irreplaceable tool in many fundamental research studies of ultrafast dynamics, the pulse generation process itself is an interesting topic in the ultrafast field. When an intense femtosecond laser is tightly focused on a gaseous target, electrons inside the neutral atoms are ripped away through tunneling ionization. Under certain circumstances, the electrons are able to reunite with the parent ions and release photon bursts lasting only tens to hundreds of attoseconds. This process repeats itself every half cycle of the driving pulse, generating a train of single attosecond pulses which lasts longer than one femtosecond. To achieve true temporal resolution on the attosecond time scale, single isolated attosecond pulses are required, meaning only one attosecond pulse can be produced per driving pulse.
Download or read book Generation of Linear Isolated Sub 60 Attosecond Pulses by Combining a Circularly Polarized Pulse with an Elliptically Polarized Pulse Supported by the National Natural Science Foundation of China Under Grant Nos 11404204 and 11447208 the Key Project of Chinese Ministry of Education Under Grant No 211025 the Research Fund for the Doctoral Program of Higher Education of China Under Grant No 20111404120004 and the Natural Science Foundation for Young Scientists of Shanxi Province Under Grant written by and published by . This book was released on 2015 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Abstract : The two-color circularly polarized pulses scheme was proposed to generate isolated attosecond pulses in our previous work [Phys. Rev. A 87 (2013) 043406 ], while the polarization of the attosecond pulse was not investigated. We show a supplementary explanation of this scheme and present another scheme to generate linear isolated attosecond pulses by combining a circularly polarized pulse with an elliptically polarized pulse. High-order harmonic generation and quantum path control are investigated to compare these two schemes. Both schemes can obtain supercontinuum spectra plateau from about 200 eV to 550 eV, which belong to the water window region. It is found that the latter scheme can clearly eliminate the short quantum path and extend the harmonic plateau. A linear isolated attosecond pulse with a duration of sub-60 as can be generated by superposing a bandwidth of 70 eV.
Download or read book High Energy and Short Pulse Lasers written by Richard Viskup and published by BoD – Books on Demand. This book was released on 2016-09-07 with total page 426 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book gives the readers an introduction to experimental and theoretical knowledge acquired by large-scale laser laboratories that are dealing with extra-high peak power and ultrashort laser pulses for research of terawatt (TW), petawatt (PW), or near-future exawatt (EW) laser interactions, for soft X-ray sources, for acceleration of particles, or for generation of hot dense thermal plasma for the laser fusion. The other part of this book is dealing with the small-scale laser laboratories that are using for its research on commercial sources of laser radiation, nanosecond (ns), picosecond (ps), or femtosecond (fs) laser pulses, either for basic research or for more advanced applications. This book is divided into six main sections dealing with short and ultrashort laser pulses, laser-produced soft X-ray sources, large-scale high-power laser systems, free-electron lasers, fiber-based sources of short optical pulse, and applications of short pulse lasers. In each chapter readers can find fascinating topics related to the high energy and/or short pulse laser technique. Individual chapters should serve the broad spectrum of readers of different expertise, layman, undergraduate and postgraduate students, scientists, and engineers, who may in this book find easily explained fundamentals as well as advanced principles of particular subjects related to these phenomena.
Download or read book Coherence and Ultrashort Pulse Laser Emission written by F. J. Duarte and published by BoD – Books on Demand. This book was released on 2010-12-30 with total page 702 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this volume, recent contributions on coherence provide a useful perspective on the diversity of various coherent sources of emission and coherent related phenomena of current interest. These papers provide a preamble for a larger collection of contributions on ultrashort pulse laser generation and ultrashort pulse laser phenomena. Papers on ultrashort pulse phenomena include works on few cycle pulses, high-power generation, propagation in various media, to various applications of current interest. Undoubtedly, Coherence and Ultrashort Pulse Emission offers a rich and practical perspective on this rapidly evolving field.
Download or read book Enhancement Cavities for the Generation of Extreme Ultraviolet and Hard X Ray Radiation written by Henning Carstens and published by Springer. This book was released on 2018-06-22 with total page 103 pages. Available in PDF, EPUB and Kindle. Book excerpt: This thesis discusses the power scaling of ultrashort pulses in enhancement cavities, utilized in particular for frequency conversion processes, such as Thomson scattering and high-harmonic generation. Using custom optics for ultrashort-pulse enhancement cavities, it demonstrates for the first time that at the envisaged power levels, the mitigation of thermal effects becomes indispensable even in cavities comprising solely reflective optics. It also studies cavities with large beams, albeit with low misalignment sensitivity, as a way to circumvent intensity-induced mirror damage. Average powers of several hundred kilowatts are demonstrated, which benefit hard x-ray sources based on Thomson scattering. Furthermore, pulses as short as 30 fs were obtained at more than 10 kW of average power and employed for high-harmonic generation with photon energies exceeding 100 eV at 250 MHz repetition rate, paving the way for frequency comb spectroscopy in this spectral region.
Download or read book Advances in Multi photon Processes and Spectroscopy written by Sheng Hsien Lin and published by World Scientific. This book was released on 2011 with total page 259 pages. Available in PDF, EPUB and Kindle. Book excerpt: In view of the rapid growth in both experimental and theoretical studies of multiphoton processes and multiphoton spectroscopy of atoms, ions and molecules in chemistry, physics, biology, materials science, etc., it is desirable to publish an Advanced Series that contains review papers readable not only by active researchers in these areas, but also by those who are not experts in the field but who intend to enter the field. The present series attempts to serve this purpose. Each review article is written in a self-contained manner by the experts in the area so that the readers can grasp the knowledge in the area without too much preparation.
Download or read book High energy Isolated Attosecond Pulses by Sub cycle Ionization Dynamics written by Federico Ferrari and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Passive Optical Resonators for Next Generation Attosecond Metrology written by Ioachim Pupeza and published by Springer Nature. This book was released on 2022 with total page 73 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book introduces readers to the development of a new generation of high pulse-repetition frequency instruments for multi-dimensional attosecond-resolution photoelectron spectroscopy (attosecond PES). It investigates the power scaling of femtosecond enhancement cavities for efficient intracavity high-harmonics generation (HHG). Further, it derives and verifies advanced resonator designs that feature large illuminated spots on all mirrors, which mitigate both intensity- and thermally-induced enhancement limitations. The dynamics of a high-finesse, passive resonator in the presence of a highly nonlinear optical process such as HHG are quantitatively investigated, both theoretically and experimentally. These investigations are instrumental in achieving the holistic optimization of the XUV source reported on here, which for the first time reached intracavity HHG conversion efficiencies comparable to those achieved in single-pass setups with a similar gas target. Coupling out the XUV beam from the enhancement cavity by purely geometric means, employing both the fundamental and higher-order transverse Gaussian modes, is studied. This offers the advantages of robustness, low distortion to the participating pulses, and photon-energy scalability. Last but not least, the author provides a range of proof-of-principle attosecond angle-resolved PES experiments. The book gives an outlook on the possible future development of cavity-enhanced HHG and an extensive discussion on the generation of isolated XUV attosecond pulses via intracavity wavefront rotation.
Download or read book Generation of Intense Isolated Attosecond Pulses at 100 EV written by Daniel E. Rivas and published by . This book was released on 2016 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Isolated Attosecond Pulses Using a Detuned Second harmonic Field written by and published by . This book was released on 2007 with total page 3 pages. Available in PDF, EPUB and Kindle. Book excerpt: Calculations are presented for the generation of an isolated attosecond pulse in a multicycle two-color strong-field regime. We show that the recollision of the electron wave packet can be confined to half an optical cycle using pulses of up to 40 fs in duration. The scheme is proven to be efficient using two intense beams, one producing a strong field at [omega] and the other a strong field detuned from 2[omega]. The slight detuning [delta][omega] of the second harmonic is used to break the symmetry of the electric field over many optical cycles and provides a coherent control for the formation of an isolated attosecond pulse.
Download or read book Advances in Atomic Molecular and Optical Physics written by Susanne Yelin and published by Academic Press. This book was released on 2020-06-17 with total page 316 pages. Available in PDF, EPUB and Kindle. Book excerpt: Advances in Atomic, Molecular, and Optical Physics, Volume 69, the latest release in this ongoing series, provides a comprehensive compilation of recent developments in a field that is in a state of rapid growth, as new experimental and theoretical techniques are used on many problems, both old and new. Topics covered in this new release include Strong-field ion spectroscopy, Configurable microscopic optical potentials, Polaritons, Rydberg excitation of trapped cold ions - a new platform for quantum technologies, High intensity QED, Recollision imaging, and more. Presents the work of international experts in the field Contains comprehensive articles that compile recent developments in a field that is experiencing rapid growth, with new experimental and theoretical techniques emerging Ideal for users interested in optics, excitons, plasmas and thermodynamics Covers atmospheric science, astrophysics, and surface and laser physics, amongst other topics
Download or read book Attosecond and XUV Physics written by Thomas Schultz and published by John Wiley & Sons. This book was released on 2013-11-13 with total page 624 pages. Available in PDF, EPUB and Kindle. Book excerpt: This book provides fundamental knowledge in the fields of attosecond science and free electron lasers, based on the insight that the further development of both disciplines can greatly benefit from mutual exposure and interaction between the two communities. With respect to the interaction of high intensity lasers with matter, it covers ultrafast lasers, high-harmonic generation, attosecond pulse generation and characterization. Other chapters review strong-field physics, free electron lasers and experimental instrumentation. Written in an easy accessible style, the book is aimed at graduate and postgraduate students so as to support the scientific training of early stage researchers in this emerging field. Special emphasis is placed on the practical approach of building experiments, allowing young researchers to develop a wide range of scientific skills in order to accelerate the development of spectroscopic techniques and their implementation in scientific experiments. The editors are managers of a research network devoted to the education of young scientists, and this book idea is based on a summer school organized by the ATTOFEL network.
Download or read book Fundamentals of Attosecond Optics written by Zenghu Chang and published by CRC Press. This book was released on 2016-04-19 with total page 536 pages. Available in PDF, EPUB and Kindle. Book excerpt: Attosecond optical pulse generation, along with the related process of high-order harmonic generation, is redefining ultrafast physics and chemistry. A practical understanding of attosecond optics requires significant background information and foundational theory to make full use of these cutting-edge lasers and advance the technology toward the n
