Download or read book Heterogeneous Nucleation of Ice on Anthropogenic Organic Particles Collected in Mexico City written by and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: This study reports on heterogeneous ice nucleation activity of predominantly organic (or coated with organic material) anthropogenic particles sampled within and around the polluted environment of Mexico City. The onset of heterogeneous ice nucleation was observed as a function of particle temperature (Tp), relative humidity (RH), nucleation mode, and particle chemical composition which is influenced by photochemical atmospheric aging. Particle analyses included computer controlled scanning electron microscopy with energy dispersive analysis of X-rays (CCSEM/EDX) and scanning transmission X-ray microscopy with near edge X-ray absorption fine structure spectroscopy (STXM/NEXAFS). In contrast to most laboratory studies employing proxies of organic aerosol, we show that anthropogenic organic particles collected in Mexico City can potentially induce ice nucleation at experimental conditions relevant to cirrus formation. The results suggest a new precedent for the potential impact of organic particles on ice cloud formation and climate.
Download or read book Chemistry In The Cryosphere In 2 Parts written by Paul Shepson and published by World Scientific. This book was released on 2021-10-12 with total page 922 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ice and snow on Earth modulate and modify the climate, chemistry and fate of air and water pollutants. Climate change is drastically impacting Nature and extent of the cryosphere, with attendant feedbacks on atmospheric composition and climate. These changes are happening at a rate that outpaces the development of fundamental knowledge of processes that occur within/on the surfaces of ice and snow, confounding our ability to develop a predictive capability for future states of the Earth environment.This set, comprising 17 chapters, written by world experts on these topics, are thus intended to document the current state of understanding of the structure, physical properties, abundance, and chemical and microbiological processes that occur within/on ice and snow in all Earth environments in which it exists, and to express needs for improvement of that understanding. This, only comprehensive treatise/collection that covers environmentally relevant chemistry and related physical aspects of snow and ice in the Earth system, and the connections to climate change, will be accessible to those with introductory college-level understanding of chemistry and physics.
Download or read book Parameterization Of Atmospheric Convection In 2 Volumes written by Robert S Plant and published by World Scientific. This book was released on 2015-08-21 with total page 1169 pages. Available in PDF, EPUB and Kindle. Book excerpt: Precipitating atmospheric convection is fundamental to the Earth's weather and climate. It plays a leading role in the heat, moisture and momentum budgets. Appropriate modelling of convection is thus a prerequisite for reliable numerical weather prediction and climate modelling. The current standard approach is to represent it by subgrid-scale convection parameterization.Parameterization of Atmospheric Convection provides, for the first time, a comprehensive presentation of this important topic. The two-volume set equips readers with a firm grasp of the wide range of important issues, and thorough coverage is given of both the theoretical and practical aspects. This makes the parameterization problem accessible to a wider range of scientists than before. At the same time, by providing a solid bottom-up presentation of convection parameterization, this set is the definitive reference point for atmospheric scientists and modellers working on such problems.Volume 1 of this two-volume set focuses on the basic principles: introductions to atmospheric convection and tropical dynamics, explanations and discussions of key parameterization concepts, and a thorough and critical exploration of the mass-flux parameterization framework, which underlies the methods currently used in almost all operational models and at major climate modelling centres. Volume 2 focuses on the practice, which also leads to some more advanced fundamental issues. It includes: perspectives on operational implementations and model performance, tailored verification approaches, the role and representation of cloud microphysics, alternative parameterization approaches, stochasticity, criticality, and symmetry constraints.
Download or read book Heterogeneous Ice Nucleation from Laboratory generated and Field collected Aerosol Particles written by Bingbing Wang and published by . This book was released on 2011 with total page 320 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Laboratory Studies of Deposition Mode Heterogeneous Ice Nucleation written by Zaminhussein Abdulali Kanji and published by . This book was released on 2009 with total page 490 pages. Available in PDF, EPUB and Kindle. Book excerpt: The indirect aerosol effect contributes to major uncertainties in determining the radiation budget of the earth. A large uncertainty is due to the formation of ice clouds onto natural or anthropogenic aerosols. Field studies have shown that mineral type particles are often associated with ice crystals in the mid-upper troposphere and given the long residence time in the atmosphere of dust particles (∼2 weeks in the absence of precipitation), their contribution to ice formation processes is not fully defined.It was concluded that there is no single value for the onset of ice formation in the atmosphere via deposition freezing. The associated contact angles show that there is a distribution of active sites on IN and that not all active sites have the same affinity for initiation of ice formation even within the same aerosol type. This work provides evidence that deposition mode nucleation can be an alternate pathway to homogeneous nucleation when mineral aerosols are present in the troposphere since the high T-low RH conditions required for deposition mode nucleation are more easily encountered in the atmosphere than the low T-high RH required for homogeneous nucleation.In order to probe ice formation onto natural mineral dust in a setting where it could be suspended as aerosol, a new continuous flow diffusion chamber (CFDC) was built. This allowed investigations of the effects of total aerosol surface area and particle size. The CFDC was also used in an international inter-comparison of ice nucleation instrumentation to compare efficiencies of soot, biological aerosol (bacteria) and samples of natural desert dusts from different regions of the world. The laboratory observations were parameterized using nucleation rates (Jhet) and contact angles (theta) as described by classical nucleation theory.For both this experimental technique and a static one developed during the candidate's Masters degree, mineral dust particulate proved to be the most efficient ice nuclei (IN) activating at RH with respect to ice (RH i) as low as 105% at T=233 K. The efficiency varied with particle size and aerosol surface area (SA). Large particles or higher SA activated at lower RHi than small particles or lower SA. The static chamber was sensitive to the first ice event out of a large SA and therefore gave true onset RHi, which was lower than the onset defined by the CFDC studies, which was not sensitive to a single ice event. In addition the static chamber used a broader size range of particulate matter, including super micron particles while the CFDC particles sizes were restricted to below 0.5 microm. Soot and organic coated dust particles were inefficient IN compared to pure dust. Soot aerosols showed some efficiency at T
Download or read book Ice Nucleation Potential and Chemical Composition of Laboratory generated and Field collected Organic Particles written by Joseph Charnawskas and published by . This book was released on 2017 with total page 77 pages. Available in PDF, EPUB and Kindle. Book excerpt:
Download or read book Experimental Investigation of Heterogeneous Nucleation of Ice in Remote Locations written by Alessia Nicosia and published by . This book was released on 2018 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: Heterogeneous ice nucleation is one element inside the overall complexity of the Earth's atmosphere, however, it has a profound impact on our representation of cloud properties: this process affects the optical thickness and lifetime of mixed-phase clouds and cirrus clouds, and it is responsible for a significant proportion of precipitations formed globally. Heterogeneous ice nucleation is related to the presence of specific aerosol particles, named ice nuclei particles (INP), with the unique ability of lowering the energy barrier required for the formation of ice crystals, especially where cloud's temperatures are >-38 °C. In the last decades, significant advancements have been made to the fundamental understanding of ice nucleation, however the lack of knowledge on the cloud ice phase still contributes to major uncertainties in climate model prediction of radiative forcing. This is partly due to limited observational data quantifying INP distributions and properties all over the world, especially in remote locations. In the first part of this thesis, field observations of ice nucleating particles have been performed at the Italian Climate Observatory “O. Vittori” on Mountain Cimone (2165 m above sea level), in the spring 2014 and autumn 2015, within the Bacchus and Air Sea Lab projects. For the first time we report the results of offline INP measurements, performed at a high altitude site within the Mediterranean basin. In the period 19-29 May 2014, a parallel campaign took place at the low-altitude station San Pietro Capofiume, a rural site in the Po Valley. The two campaigns were concerned, for a few days, by a Saharan Dust transport Event, which was recorded simultaneously at the high and the low-level station. We investigated the ambient number concentration of INP under condensation freezing activation mechanism (at -18 °C and above water saturation). In the second part of this thesis, we present the observations that were performed during the Arctic campaign Parcs-Maca, in the period of transition among the polar night and the polar day. We could characterise for the first time the ice nucleating and physical/chemical properties of the Arctic Primary Marine Aerosol, in a laboratory-controlled generation approach, that was combined to a mesocosm experiment. The aim of the mesocosm experiment was to adopt a multidisciplinary approach to study the effect of marine pollution on marine emissions. We found a moderate but significant decrease of the ice nuclei concentration in the polluted seawater (with respect to the control seawater) recorded in the freezing range between -8.5 and -19 °C and activated through immersion-freezing. Within the seaspray our measurements have indicated a relation among INP active at warm temperature (above -15 °C through immersion-freezing) and a calcium enrichment detected in PM1 filters (and followed by an apparent Chloride depletion). On the basis of our observations, and the results reported from other studies, a few suggestions on the nature of these marine ice nuclei have been suggested. In summary, the measurements made for this thesis provide new information on the concentrations of ice nuclei in ambient aerosol particles in remote regions (a high-altitude observatory in the central Mediterranean region) and in relation to a specific source (the Arctic sea spray).
Download or read book Light Scattering by Ice Crystals written by Kuo-Nan Liou and published by Cambridge University Press. This book was released on 2016-10-06 with total page 461 pages. Available in PDF, EPUB and Kindle. Book excerpt: This volume outlines the fundamentals and applications of light scattering, absorption and polarization processes involving ice crystals.
Download or read book Atmospheric Aerosols written by Claudio Tomasi and published by John Wiley & Sons. This book was released on 2017-03-20 with total page 706 pages. Available in PDF, EPUB and Kindle. Book excerpt: Ein Blick auf die morphologischen, physikalischen und chemischen Eigenschaften von Aerosolen aus den unterschiedlichsten natürlichen und anthropogenen Quellen trägt zum besseren Verständnis der Rolle bei, die Aerosolpartikel bei der Streuung und Absorption kurz- und langwelliger Strahlung spielen. Dieses Fachbuch bietet Informationen, die sonst schwer zu finden sind, und vermittelt ausführlich die Kenntnisse, die erforderlich sind, um die mikrophysikalischen, chemischen und Strahlungsparameter zu charakterisieren, die bei der Wechselwirkung von Sonnen- und Erdstrahlen so überaus wichtig sind. Besonderes Augenmerk liegt auf den indirekten Auswirkungen von Aerosolen auf das Klima im Rahmen des komplexen Systems aus Aerosolen, Wolken und der Atmosphäre. Auch geht es vorrangig um die Wirkungen natürlicher und anthropogener Aerosole auf die Luftqualität und die Umwelt, auf die menschliche Gesundheit und unser kulturelles Erbe. Mit einem durchgängig lösungsorientierten Ansatz werden nicht nur die Probleme und Gefahren dieser Aerosole behandelt, sondern auch praktikable Lösungswege aufgezeigt.
Download or read book Microphysics of Clouds and Precipitation written by H.R. Pruppacher and published by Springer Science & Business Media. This book was released on 2010-06-25 with total page 975 pages. Available in PDF, EPUB and Kindle. Book excerpt: Cloud physics has achieved such a voluminous literature over the past few decades that a significant quantitative study of the entire field would prove unwieldy. This book concentrates on one major aspect: cloud microphysics, which involves the processes that lead to the formation of individual cloud and precipitation particles. Common practice has shown that one may distinguish among the following addi tional major aspects: cloud dynamics, which is concerned with the physics respon sible for the macroscopic features of clouds; cloud electricity, which deals with the electrical structure of clouds and the electrification processes of cloud and precipi tation particles; and cloud optics and radar meteorology, which describe the effects of electromagnetic waves interacting with clouds and precipitation. Another field intimately related to cloud physics is atmospheric chemistry, which involves the chemical composition ofthe atmosphere and the life cycle and characteristics of its gaseous and particulate constituents. In view of the natural interdependence of the various aspects of cloud physics, the subject of microphysics cannot be discussed very meaningfully out of context. Therefore, we have found it necessary to touch briefly upon a few simple and basic concepts of cloud dynamics and thermodynamics, and to provide an account of the major characteristics of atmospheric aerosol particles. We have also included a separate chapter on some of the effects of electric fields and charges on the precipitation-forming processes.
Download or read book An Introduction to Clouds written by Ulrike Lohmann and published by Cambridge University Press. This book was released on 2016-06-23 with total page 419 pages. Available in PDF, EPUB and Kindle. Book excerpt: An Introduction to Clouds provides a fundamental understanding of clouds, ranging from cloud microphysics to the large-scale impacts of clouds on climate. On the microscale, phase changes and ice nucleation are covered comprehensively, including aerosol particles and thermodynamics relevant for the formation of clouds and precipitation. At larger scales, cloud dynamics, mid-latitude storms and tropical cyclones are discussed leading to the role of clouds on the hydrological cycle and climate. Each chapter ends with problem sets and multiple-choice questions that can be completed online, and important equations are highlighted in boxes for ease of reference. Combining mathematical formulations with qualitative explanations of underlying concepts, this accessible book requires relatively little previous knowledge, making it ideal for advanced undergraduate and graduate students in atmospheric science, environmental sciences and related disciplines.
Download or read book Climate Change 2013 The Physical Science Basis written by Intergouvernemental panel on climate change. Working group 1 and published by Cambridge University Press. This book was released on 2014 with total page 1553 pages. Available in PDF, EPUB and Kindle. Book excerpt: The report also provides a comprehensive assessment of past and future sea level change in a dedicated chapter.
Download or read book Aerosol Pollution Impact on Precipitation written by Zev Levin and published by Springer Science & Business Media. This book was released on 2008-09-30 with total page 399 pages. Available in PDF, EPUB and Kindle. Book excerpt: Life on Earth is critically dependent upon the continuous cycling of water between oceans, continents and the atmosphere. Precipitation (including rain, snow, and hail) is the primary mechanism for transporting water from the atmosphere back to the Earth’s surface. It is also the key physical process that links aspects of climate, weather, and the global hydrological cycle. Changes in precipitation regimes and the frequency of extreme weather events, such as floods, droughts, severe ice/snow storms, monsoon fluctuations and hurricanes are of great potential importance to life on the planet. One of the factors that could contribute to precipitation modification is aerosol pollution from various sources such as urban air pollution and biomass burning. Natural and anthropogenic changes in atmospheric aerosols might have important implications for precipitation by influencing the hydrological cycle, which in turn could feed back to climate changes. From an Earth Science perspective, a key question is how changes expected in climate will translate into changes in the hydrological cycle, and what trends may be expected in the future. We require a much better understanding and hence predictive capability of the moisture and energy storages and exchanges among the Earth’s atmosphere, oceans, continents and biological systems. This book is a review of our knowledge of the relationship between aerosols and precipitation reaching the Earth's surface and it includes a list of recommendations that could help to advance our knowledge in this area.
Download or read book Atmospheric Physics written by Ulrich Schumann and published by Springer Science & Business Media. This book was released on 2012-07-17 with total page 884 pages. Available in PDF, EPUB and Kindle. Book excerpt: On the occasion of the 50th anniversary of the Institute of Atmospheric Physics of the German Aerospace Center (DLR), this book presents more than 50 chapters highlighting results of the institute’s research. The book provides an up-to-date, in-depth survey across the entire field of atmospheric science, including atmospheric dynamics, radiation, cloud physics, chemistry, climate, numerical simulation, remote sensing, instruments and measurements, as well as atmospheric acoustics. The authors have provided a readily comprehensible and self-contained presentation of the complex field of atmospheric science. The topics are of direct relevance for aerospace science and technology. Future research challenges are identified.
Download or read book Outdoor Air Pollution written by IARC Working Group on the Evaluation of Carcinogenic Risks to Humans and published by IARC Monographs on the Evaluat. This book was released on 2016 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: "This publication represents the views and expert opinions of an IARC Working Group on the Evaluation of Carcinogenic Risk to Humans, which met in Lyon, 8-15 October 2013."
Download or read book Aerosol Science written by Ian Colbeck and published by John Wiley & Sons. This book was released on 2014-02-03 with total page 522 pages. Available in PDF, EPUB and Kindle. Book excerpt: AEROSOL SCIENCE TECHNOLOGY AND APPLICATIONS Aerosols influence many areas of our daily life. They are at the core of environmental problems such as global warming, photochemical smog and poor air quality. They can also have diverse effects on human health, where exposure occurs in both outdoor and indoor environments. However, aerosols can have beneficial effects too; the delivery of drugs to the lungs, the delivery of fuels for combustion and the production of nanomaterials all rely on aerosols. Advances in particle measurement technologies have made it possible to take advantage of rapid changes in both particle size and concentration. Likewise, aerosols can now be produced in a controlled fashion. Reviewing many technological applications together with the current scientific status of aerosol modelling and measurements, this book includes: Satellite aerosol remote sensing The effects of aerosols on climate change Air pollution and health Pharmaceutical aerosols and pulmonary drug delivery Bioaerosols and hospital infections Particle emissions from vehicles The safety of emerging nanomaterials Radioactive aerosols: tracers of atmospheric processes With the importance of this topic brought to the public's attention after the eruption of the Icelandic volcano Eyjafjallajökull, this book provides a timely, concise and accessible overview of the many facets of aerosol science.
Download or read book Climate Change 2013 The Physical Science Basis written by Intergovernmental Panel on Climate Change (IPCC) and published by Cambridge University Press. This book was released on 2014-03-24 with total page 1554 pages. Available in PDF, EPUB and Kindle. Book excerpt: This Fifth Assessment Report of the Intergovernmental Panel on Climate Change (IPCC) will again form the standard scientific reference for all those concerned with climate change and its consequences, including students and researchers in environmental science, meteorology, climatology, biology, ecology and atmospheric chemistry. It provides invaluable material for decision makers and stakeholders at international, national and local level, in government, businesses, and NGOs. This volume provides: • An authoritative and unbiased overview of the physical science basis of climate change • A more extensive assessment of changes observed throughout the climate system than ever before • New dedicated chapters on sea-level change, biogeochemical cycles, clouds and aerosols, and regional climate phenomena • Extensive coverage of model projections, both near-term and long-term climate projections • A detailed assessment of climate change observations, modelling, and attribution for every continent • A new comprehensive atlas of global and regional climate projections for 35 regions of the world
