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Book Fuel Tracer Photophysics for Quantitative Planar Laser induced Fluorescence

Download or read book Fuel Tracer Photophysics for Quantitative Planar Laser induced Fluorescence written by Jon Koch and published by . This book was released on 2005 with total page 143 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Tracer based Planar Laser induced Fluorescence Diagnostics

Download or read book Tracer based Planar Laser induced Fluorescence Diagnostics written by Brian Ho-yin Cheung and published by Stanford University. This book was released on 2011 with total page 197 pages. Available in PDF, EPUB and Kindle. Book excerpt: Two advances to tracer-based planar laser-induced fluorescence (PLIF) diagnostics are presented in this work. The first improvement is the development of a 3-pentanone fluorescence quantum yield (FQY) database and model for a wide range of conditions in support of quantitative PLIF diagnostics. In addition, this work presents a sensitive, time-resolved tracer-based PLIF diagnostic, accomplished by using a continuous-wave (CW) laser with the high-FQY tracer toluene. Because of its ease of use and desirable photophysical properties, PLIF diagnostics using 3-pentanone as a tracer are common, particularly for internal combustion engine (ICE) diagnostics. Thus, there is a need for 3-pentanone FQY measurements and modeling over a wide range of temperatures, pressures, and excitation wavelengths. For insight into the collisionless process in the FQY model, measurements were made in 3-pentanone vapor at low-pressures across a range of temperatures using a flowing cell. Laser excitation with 248, 266, 277, 308 nm wavelengths were utilized, and Rayleigh scattering of the laser beam was used to calibrate the optical efficiency of the collection optics and detector. This low-pressure data allows calculation of the 3-pentanone fluorescence rate and non-radiative de-excitation rate in the fluorescence model. The vibrational relaxation cascade parameter for 3-pentanone collisions was also determined. Measurements of 3-pentanone FQY were also made over a range of temperatures and pressures relevant to diagnostic applications, and, in particular, combined high-temperature and high-pressure conditions applicable to internal combustion engines (ICE). These data were collected in a custom-built optical cell capable of simultaneous high-pressure and high-temperature conditions. The behavior of the FQY in nitrogen for temperatures up to 745 K and in air up to 570 K was examined for pressures from 1 to 25 bar. These data were used to further optimize the parameters in the FQY model representing collisional processes. The large quantity of data with 308 nm excitation allowed optimization of the nitrogen quenching rate, and data in air were used to optimize the oxygen quenching rate. These data were also used to optimize the vibrational relaxation parameters for nitrogen and oxygen. The model with the updated parameters is consistent with the data collected in the current work, as well as with fluorescence measurements made in optical ICEs up to 1100 K and 28 bar. Another area of tracer-based PLIF diagnostics development is time-resolved imaging. Because PLIF diagnostics are often performed using pulsed lasers, the time resolution of measurements is limited to the pulse rate of laser. Use of a high-powered visible laser with an off-the-shelf cavity frequency doubler is shown to produce a moderate-power CW beam in the ultraviolet wavelength regime. Application of this CW source to excite toluene, a high-FQY tracer, yields a sensitive, time-resolved tracer-based PLIF diagnostic. Fluctuation detection limits for tracer mole fraction were investigated by applying the diagnostic to an atmospheric temperature and pressure nitrogen jet seeded with 4% toluene, and detection limits of better than 1% of the maximum toluene mole fraction were achieved for detection of fluorescence signal at a point, along a line, and over a plane. The diagnostic was also demonstrated on a turbulent jet for line and planar detection and demonstrated the potential for toluene time-resolved PLIF diagnostics with CW lasers.

Book Tracer based Planar Laser induced Fluorescence Diagnostics

Download or read book Tracer based Planar Laser induced Fluorescence Diagnostics written by Brian Ho-yin Cheung and published by . This book was released on 2011 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Two advances to tracer-based planar laser-induced fluorescence (PLIF) diagnostics are presented in this work. The first improvement is the development of a 3-pentanone fluorescence quantum yield (FQY) database and model for a wide range of conditions in support of quantitative PLIF diagnostics. In addition, this work presents a sensitive, time-resolved tracer-based PLIF diagnostic, accomplished by using a continuous-wave (CW) laser with the high-FQY tracer toluene. Because of its ease of use and desirable photophysical properties, PLIF diagnostics using 3-pentanone as a tracer are common, particularly for internal combustion engine (ICE) diagnostics. Thus, there is a need for 3-pentanone FQY measurements and modeling over a wide range of temperatures, pressures, and excitation wavelengths. For insight into the collisionless process in the FQY model, measurements were made in 3-pentanone vapor at low-pressures across a range of temperatures using a flowing cell. Laser excitation with 248, 266, 277, 308 nm wavelengths were utilized, and Rayleigh scattering of the laser beam was used to calibrate the optical efficiency of the collection optics and detector. This low-pressure data allows calculation of the 3-pentanone fluorescence rate and non-radiative de-excitation rate in the fluorescence model. The vibrational relaxation cascade parameter for 3-pentanone collisions was also determined. Measurements of 3-pentanone FQY were also made over a range of temperatures and pressures relevant to diagnostic applications, and, in particular, combined high-temperature and high-pressure conditions applicable to internal combustion engines (ICE). These data were collected in a custom-built optical cell capable of simultaneous high-pressure and high-temperature conditions. The behavior of the FQY in nitrogen for temperatures up to 745 K and in air up to 570 K was examined for pressures from 1 to 25 bar. These data were used to further optimize the parameters in the FQY model representing collisional processes. The large quantity of data with 308 nm excitation allowed optimization of the nitrogen quenching rate, and data in air were used to optimize the oxygen quenching rate. These data were also used to optimize the vibrational relaxation parameters for nitrogen and oxygen. The model with the updated parameters is consistent with the data collected in the current work, as well as with fluorescence measurements made in optical ICEs up to 1100 K and 28 bar. Another area of tracer-based PLIF diagnostics development is time-resolved imaging. Because PLIF diagnostics are often performed using pulsed lasers, the time resolution of measurements is limited to the pulse rate of laser. Use of a high-powered visible laser with an off-the-shelf cavity frequency doubler is shown to produce a moderate-power CW beam in the ultraviolet wavelength regime. Application of this CW source to excite toluene, a high-FQY tracer, yields a sensitive, time-resolved tracer-based PLIF diagnostic. Fluctuation detection limits for tracer mole fraction were investigated by applying the diagnostic to an atmospheric temperature and pressure nitrogen jet seeded with 4% toluene, and detection limits of better than 1% of the maximum toluene mole fraction were achieved for detection of fluorescence signal at a point, along a line, and over a plane. The diagnostic was also demonstrated on a turbulent jet for line and planar detection and demonstrated the potential for toluene time-resolved PLIF diagnostics with CW lasers.

Book Strategies for Planar Laser induced Fluorescence Thermometry in Shock Tube Flows

Download or read book Strategies for Planar Laser induced Fluorescence Thermometry in Shock Tube Flows written by Ji Hyung Yoo and published by Stanford University. This book was released on 2011 with total page 151 pages. Available in PDF, EPUB and Kindle. Book excerpt: This thesis was motivated by the need to better understand the temperature distribution in shock tube flows, especially in the near-wall flow regions. Two main ideas in planar laser-induced fluorescence (PLIF) diagnostics are explored in this thesis. The first topic is the development of a single-shot PLIF diagnostic technique for quantitative temperature distribution measurement in shock tube flow fields. PLIF is a non-intrusive, laser-based diagnostic technique capable of instantaneously imaging key flow features, such as temperature, pressure, density, and species concentration, by measuring fluorescence signal intensity from laser-excited tracer species. This study performed a comprehensive comparison of florescence tracers and excitation wavelengths to determine the optimal combination for PLIF imaging in shock tube flow applications. Excitation of toluene at 248nm wavelength was determined to be the optimal strategy due to the resulting high temperature sensitivity and fluorescence signal level, compared to other ketone and aromatic tracers at other excitation wavelengths. Sub-atmospheric toluene fluorescence yield data was measured to augment the existing photophysical data necessary for this diagnostic technique. In addition, a new imaging test section was built to allow PLIF imaging in all regions of the shock tube test section, including immediately adjacent to the side and end walls. The signal-to-noise (SNR) and spatial resolution of the PLIF images were optimized using statistical analysis. Temperature field measurements were made with the PLIF diagnostic technique across normal incident and reflected shocks in the shock tube core flow. The resulting images show uniform spatial distribution, and good agreement with conditions calculated from the normal shock jump equations. Temperature measurement uncertainty is about 3.6% at 800K. The diagnostic was also applied to image flow over a wedge. The resulting images capture all the flow features predicted by numerical simulations. The second topic is the development of a quantitative near-wall diagnostic using tracer-based PLIF imaging. Side wall thermal boundary layers and end wall thermal layers are imaged to study the temperature distribution present under constant pressure conditions. The diagnostic technique validated in the shock tube core flow region was further optimized to improve near-wall image quality. The optimization process considered various wall materials, laser sheet orientations, camera collection angles, and optical components to find the configuration that provides the best images. The resulting images have increased resolution (15[Mu]m) and are able to resolve very thin non-uniform near-wall temperature layers (down to 60[Mu]m from the surface). The temperature field and thickness measurements of near-wall shock tube flows under various shock conditions and test gases showed good agreement with boundary layer theory. To conclude this thesis, new applications and future improvements to the developed PLIF diagnostic technique are discussed. These suggested refinements can provide an even more robust and versatile PLIF imaging technique capable of measuring a wider range of flow conditions near walls.

Book Quantitative Plif Imaging in High Pressure Combustion

Download or read book Quantitative Plif Imaging in High Pressure Combustion written by National Aeronautics and Space Adm Nasa and published by Independently Published. This book was released on 2018-11-06 with total page 64 pages. Available in PDF, EPUB and Kindle. Book excerpt: This is the final report for a research project aimed at developing planar laser-induced fluorescence (PLIF) techniques for quantitative 2-D species imaging in fuel-lean, high-pressure combustion gases, relevant to modem aircraft gas turbine combustors. The program involved both theory and experiment. The theoretical activity led to spectroscopic models that allow calculation of the laser-induced fluorescence produced in OH, NO and 02 for arbitrary excitation wavelength, pressure, temperature, gas mixture and laser linewidth. These spectroscopic models incorporate new information on line- broadening, energy transfer and electronic quench rates. Extensive calculations have been made with these models in order to identify optimum excitation strategies, particularly for detecting low levels (ppm) of NO in the presence of large 02 mole fractions (10% is typical for the fuel-lean combustion of interest). A promising new measurement concept has emerged from these calculations, namely that excitation at specific wavelengths, together with detection of fluorescence in multiple spectral bands, promises to enable simultaneous detection of both NO (at ppm levels) and 02 or possibly NO, 02 and temperature. Calculations have been made to evaluate the expected performance of such a diagnostic for a variety of conditions and choices of excitation and detection wavelengths. The experimental effort began with assembly of a new high-pressure combustor to provide controlled high-temperature and high-pressure combustion products. The non-premixed burner enables access to postflame gases at high temperatures (to 2000 K) and high pressures (to 13 atm), and a range of fuel-air equivalence ratios. The chamber also allowed use of a sampling probe, for chemiluminescent detection of NO/NO2, and thermocouples for measurement of gas temperature. Experiments were conducted to confirm the spectroscopic models for OH, NO and 02. Hanson, R. K. Glenn Research Center...

Book Strategies for Planar Laser induced Fluorescence Thermometry in Shock Tube Flows

Download or read book Strategies for Planar Laser induced Fluorescence Thermometry in Shock Tube Flows written by Ji Hyung Yoo and published by . This book was released on 2011 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: This thesis was motivated by the need to better understand the temperature distribution in shock tube flows, especially in the near-wall flow regions. Two main ideas in planar laser-induced fluorescence (PLIF) diagnostics are explored in this thesis. The first topic is the development of a single-shot PLIF diagnostic technique for quantitative temperature distribution measurement in shock tube flow fields. PLIF is a non-intrusive, laser-based diagnostic technique capable of instantaneously imaging key flow features, such as temperature, pressure, density, and species concentration, by measuring fluorescence signal intensity from laser-excited tracer species. This study performed a comprehensive comparison of florescence tracers and excitation wavelengths to determine the optimal combination for PLIF imaging in shock tube flow applications. Excitation of toluene at 248nm wavelength was determined to be the optimal strategy due to the resulting high temperature sensitivity and fluorescence signal level, compared to other ketone and aromatic tracers at other excitation wavelengths. Sub-atmospheric toluene fluorescence yield data was measured to augment the existing photophysical data necessary for this diagnostic technique. In addition, a new imaging test section was built to allow PLIF imaging in all regions of the shock tube test section, including immediately adjacent to the side and end walls. The signal-to-noise (SNR) and spatial resolution of the PLIF images were optimized using statistical analysis. Temperature field measurements were made with the PLIF diagnostic technique across normal incident and reflected shocks in the shock tube core flow. The resulting images show uniform spatial distribution, and good agreement with conditions calculated from the normal shock jump equations. Temperature measurement uncertainty is about 3.6% at 800K. The diagnostic was also applied to image flow over a wedge. The resulting images capture all the flow features predicted by numerical simulations. The second topic is the development of a quantitative near-wall diagnostic using tracer-based PLIF imaging. Side wall thermal boundary layers and end wall thermal layers are imaged to study the temperature distribution present under constant pressure conditions. The diagnostic technique validated in the shock tube core flow region was further optimized to improve near-wall image quality. The optimization process considered various wall materials, laser sheet orientations, camera collection angles, and optical components to find the configuration that provides the best images. The resulting images have increased resolution (15[Mu]m) and are able to resolve very thin non-uniform near-wall temperature layers (down to 60[Mu]m from the surface). The temperature field and thickness measurements of near-wall shock tube flows under various shock conditions and test gases showed good agreement with boundary layer theory. To conclude this thesis, new applications and future improvements to the developed PLIF diagnostic technique are discussed. These suggested refinements can provide an even more robust and versatile PLIF imaging technique capable of measuring a wider range of flow conditions near walls.

Book Annual Research Briefs

Download or read book Annual Research Briefs written by Center for Turbulence Research (U.S.) and published by . This book was released on 2011 with total page 434 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Quantitative Planar Laser Induced Fluorescence Technology

Download or read book Quantitative Planar Laser Induced Fluorescence Technology written by Zhen Yang and published by . This book was released on 2019 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: Planar laser-induced fluorescence (PLIF) is a highly sensitive and space-time-resolved laser diagnostic technique. It is widely used in the diagnosis of combustion and flow fields to obtain the thermodynamic information of active components and interested molecules in flames. Nowadays, the PLIF technology is developing in two directions: high speed and quantification. In view of the high spatial and temporal resolution characteristics of PLIF technology that other laser diagnostics do not possess, this chapter will focus on the basic principle of laser-induced fluorescence and the current research status of quantitative PLIF technology. In addition, the advantages and disadvantages of various quantitative technologies of component concentration in flames based on laser-induced fluorescence technology are analyzed. At last, the latest works on the quantification of species concentration using planar laser-induced fluorescence in combustion are introduced.

Book Planar Laser Induced Fluorescence as a Diagnostic for Determining Mass Distribution in Gas Puff PRS Loads

Download or read book Planar Laser Induced Fluorescence as a Diagnostic for Determining Mass Distribution in Gas Puff PRS Loads written by and published by . This book was released on 2003 with total page 0 pages. Available in PDF, EPUB and Kindle. Book excerpt: In this work we report on our efforts to develop a laser induced fluorescence system (LIF), using nitric oxide (NO) as the tracer, to determine the mass distribution in a gas puff nozzle assembly used as a z-pinch plasma radiation source load. The same assembly has also been extensively studied at NRL using laser interferometry at Titan, Pulsed Sciences Division using LIF with acetone as the tracer. Preliminary results indicate that the NO-LIF, laser interferometry and the previous LIF results agree to within 20%. Concentrations of NO less than 0.1% can be used.

Book Laser Based Flowfield Imaging in a Lean Premixed Prevaporized Sector Combustor

Download or read book Laser Based Flowfield Imaging in a Lean Premixed Prevaporized Sector Combustor written by National Aeronautics and Space Administration (NASA) and published by Createspace Independent Publishing Platform. This book was released on 2018-06 with total page 74 pages. Available in PDF, EPUB and Kindle. Book excerpt: OH and fuel planar laser-induced fluorescence (PLIF) is used qualitatively in this study to observe the flame structure resultant from different fuel injector dome configurations within the 3-cup sector combustor test rig. The fluorescence images are compared with some computational fluid dynamics (CFD) results. Interferences in obtaining OH fluorescence signals due to the emission of other species are assessed. NO PLIF images are presented and compared to gas analysis results. The comparison shows that PLIF NO can be an excellent method for measuring NO in the flame. Additionally, we present flow visualization of the molecular species C2.Hicks, Yolanda R. and Locke, Randy J. and Anderson, Robert C.Glenn Research CenterCOMPUTATIONAL FLUID DYNAMICS; FLOW DISTRIBUTION; LASER INDUCED FLUORESCENCE; PREMIXING; COMBUSTION CHAMBERS; PREVAPORIZATION; GAS ANALYSIS; FUEL INJECTION; DETECTORS; CCD CAMERAS; LASER BEAMS; HYDROXIDES; NITROGEN OXIDES; IMAGE ANALYSIS; LASER APPLICATIONS

Book Excitation detection strategies for OH planar laser induced fluorescence measurements in the presence of interfering fuel signal and absorption effects

Download or read book Excitation detection strategies for OH planar laser induced fluorescence measurements in the presence of interfering fuel signal and absorption effects written by and published by . This book was released on 2011 with total page 19 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Quantitative Imaging of Turbulent Gaseous Jets Using Planar Laser induced Fluorescence

Download or read book Quantitative Imaging of Turbulent Gaseous Jets Using Planar Laser induced Fluorescence written by Ike Van Cruyningen and published by Ann Arbor, Mich. : University Microfilms International. This book was released on 1990 with total page 244 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Laser Induced Fluorescence Gas Puff Density Measurements

Download or read book Laser Induced Fluorescence Gas Puff Density Measurements written by Matthew Thomas Evans and published by . This book was released on 2012 with total page 122 pages. Available in PDF, EPUB and Kindle. Book excerpt: The double gas puff valve is a device used to inject a supersonic puff of gas to act as a load in z-pinch plasma implosions. The purpose of the annular gas shells is to mimic a cylindrical column along the z-axis in efforts to reduce Rayleigh-Taylor instability. However before integration of the valve into the zpinch pulsed power machine the gas profile needs to be examined. Tuning the density of the gas to fit specific profiles leads to improvement in plasma radiative sources and yields. The axial uniformity of the cylindrical gas column is highly dependent on the nozzle characteristics and shape. Performance is then determined by the density, speed, and symmetry of the gas column. Measurement of the density distribution is performed using a spectroscopic measuring technique called laser-induced fluorescence. LIF is a 1-dimensional imaging technique that maps the concentration of atoms with the aid of a tracer. LIF and the 2-dimensional counterpart planar laser-induced fluorescence (PLIF) examine the gas flow in the r-z plane with sub-millimeter resolution. The tracer molecule fluoresces due to excitation by a laser beam. The fluorescence signal is imaged using a streak camera and a charge-coupled-device (CCD) in combination. The method also allows the study of gas puff reliability. Any differences between gas shells can then be examined and interpreted with reliable certainty. Imaging software is used to determine the density from the intensity of the fluorescence images. A detail account of the process is illustrated in this study. A control system was constructed for operations of the gas puff valve in both LIF and z-pinch experiments. The pressure system is designed to tailor specific profiles as needed. The LIF system is detailed along with any components built for the gas puff valve. Results of these measurements serve to verify the uniformity of flow and determine the density distribution of the gas puff.

Book Advanced Diagnostics for Reacting Flows

Download or read book Advanced Diagnostics for Reacting Flows written by and published by . This book was released on 2006 with total page 4 pages. Available in PDF, EPUB and Kindle. Book excerpt: Recent advances in this program's research and development of non-intrusive diagnostics for air-breathing combustion applications are reported. Progress is highlighted on: the validation of infrared-planar laser induced fluorescence (IR-PLIF) models for quantitative CO2 detection; quantitative NO PLIF in high-pressure flames; increased tunable diode laser (TDL) absorption sensor temperature fidelity in scramjet flowfields using wavelength-modulation techniques; differential-absorption with novel new light sources in the mid-IR for fuel sensing; use of wavelength-multiplexed TDL sensing for gas temperature in non-uniform flow fields; and advances in toluene photophysics to enable tracer-based PLIF imaging of temperature fields.

Book Quantitative Measurement of 2 D Fuel Vapor Concentration in a Transient Spray Via Laser induced Fluorescence Technique

Download or read book Quantitative Measurement of 2 D Fuel Vapor Concentration in a Transient Spray Via Laser induced Fluorescence Technique written by Chi-Nan Yeh and published by . This book was released on 1994 with total page 12 pages. Available in PDF, EPUB and Kindle. Book excerpt: