EBookClubs

Read Books & Download eBooks Full Online

EBookClubs

Read Books & Download eBooks Full Online

Book Development of Techniques for Spent Fuel Assay   Differential Dieaway Final Report

Download or read book Development of Techniques for Spent Fuel Assay Differential Dieaway Final Report written by and published by . This book was released on 2016 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: This report summarizes the work done under a DNDO R & D funded project on the development of the differential dieaway method to measure plutonium in spent fuel. There are large amounts of plutonium that are contained in spent fuel assemblies and currently there is no way to make quantitative non-destructive assay. This has led NA24 under the Next Generation Safeguards Initiative (NGSI) to establish a multi-year program to investigate, develop and implement measurement techniques for spent fuel [1, 2, 3]. The techniques which are being experimentally tested by the existing NGSI project do not include any pulsed neutron active techniques. The present work covers the active neutron differential dieaway technique and has advanced the state of knowledge of this technique as well as produced a design for a practical active neutron interrogation instrument for spent fuel. Monte Carlo results from the NGSI effort show that much higher accuracy (1-2%) for the Pu content in spent fuel assemblies can be obtained with active neutron interrogation techniques [4, 5] than passive techniques and this would allow their use for nuclear material accountancy independently of any information from the operator. The main purpose of this work was to develop an active neutron interrogation technique for spent nuclear fuel.

Book Utilization of the Differential Die Away Self Interrogation Technique for Characterization and Verification of Spent Nuclear Fuel

Download or read book Utilization of the Differential Die Away Self Interrogation Technique for Characterization and Verification of Spent Nuclear Fuel written by and published by . This book was released on 2016 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: New nondestructive assay techniques are sought to better characterize spent nuclear fuel. One of the NDA instruments selected for possible deployment is differential die-away self-interrogation (DDSI). The proposed DDSI approach for spent fuel assembly assay utilizes primarily the spontaneous fission and ([alpha], n) neutrons in the assemblies as an internal interrogating radiation source. The neutrons released in spontaneous fission or ([alpha], n) reactions are thermalized in the surrounding water and induce fission in fissile isotopes, thereby creating a measurable signal from isotopes of interest that would be otherwise difficult to measure. The DDSI instrument employs neutron coincidence counting with 3He tubes and list-mode-based data acquisition to allow for production of Rossi-alpha distributions (RADs) in post-processing. The list-mode approach to data collection and subsequent construction of RADs has expanded the analytical possibilities, as will be demonstrated throughout this thesis. One of the primary advantages is that the measured signal in the form of a RAD can be analyzed in its entirety including determination of die-away times in different time domains. This capability led to the development of the early die-away method, a novel leakage multiplication determination method which is tested throughout the thesis on different sources in simulation space and fresh fuel experiments. The early die-away method is a robust, accurate, improved method of determining multiplication without the need for knowledge of the ([alpha], n) source term. The DDSI technique and instrument are presented along with the many novel capabilities enabled by and discovered through RAD analysis. Among the new capabilities presented are the early die-away method, total plutonium content determination, and highly sensitive missing pin detection. Simulation of hundreds of different spent and fresh fuel assemblies were used to develop the analysis algorithms and the techniques were tested on a variety of spontaneous fission-driven fresh fuel assemblies at Los Alamos National Laboratory and the BeRP ball at the Nevada National Security Site. The development of the new, improved analysis and characterization methods with the DDSI instrument makes it a viable technique for implementation in a facility to meet material control and safeguards needs.

Book Nondestructive Verification and Assay Systems for Spent Fuels  Technical Appendixes

Download or read book Nondestructive Verification and Assay Systems for Spent Fuels Technical Appendixes written by and published by . This book was released on 1982 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Six technical appendixes are presented that provide important supporting technical information for the study of the application of nondestructive measurements to spent-fuel storage. Each appendix addresses a particular technical subject in a reasonably self-contained fashion. Appendix A is a comparison of spent-fuel data predicted by reactor operators with measured data from reprocessors. This comparison indicates a rather high level of uncertainty in previous burnup calculations. Appendix B describes a series of nondestructive measurements at the GE-Morris Operation Spent-Fuel Storage Facility. This series of experiments successfully demonstrated a technique for reproducible positioning of fuel assemblies for nondestructive measurement. The experimental results indicate the importance of measuring the axial and angular burnup profiles of irradiated fuel assemblies for quantitative determination of spent-fuel parameters. Appendix C is a reasonably comprehensive bibliography of reports and symposia papers on spent-fuel nondestructive measurements to April 1981. Appendix D is a compendium of spent-fuel calculations that includes isotope production and depletion calculations using the EPRI-CINDER code, calculations of neutron and gamma-ray source terms, and correlations of these sources with burnup and plutonium content. Appendix E describes the pulsed-neutron technique and its potential application to spent-fuel measurements. Although not yet developed, the technique holds the promise of providing separate measurements of the uranium and plutonium fissile isotopes. Appendix F describes the experimental program and facilities at Los Alamos for the development of spent-fuel nondestructive measurement systems. Measurements are reported showing that the active neutron method is sensitive to the replacement of a single fuel rod with a dummy rod in an unirradiated uranium fuel assembly.

Book Development of Techniques for Spent Fuel Assay  u2013  Differential Dieaway Final Report

Download or read book Development of Techniques for Spent Fuel Assay u2013 Differential Dieaway Final Report written by and published by . This book was released on 2016 with total page 34 pages. Available in PDF, EPUB and Kindle. Book excerpt: This report summarizes the work done under a DNDO R&D funded project on the development of the differential dieaway method to measure plutonium in spent fuel. There are large amounts of plutonium that are contained in spent fuel assemblies, and currently there is no way to make quantitative non-destructive assay. This has led NA24 under the Next Generation Safeguards Initiative (NGSI) to establish a multi-year program to investigate, develop and implement measurement techniques for spent fuel. The techniques which are being experimentally tested by the existing NGSI project do not include any pulsed neutron active techniques. The present work covers the active neutron differential dieaway technique and has advanced the state of knowledge of this technique as well as produced a design for a practical active neutron interrogation instrument for spent fuel. Monte Carlo results from the NGSI effort show that much higher accuracy (1-2%) for the Pu content in spent fuel assemblies can be obtained with active neutron interrogation techniques than passive techniques, and this would allow their use for nuclear material accountancy independently of any information from the operator. The main purpose of this work was to develop an active neutron interrogation technique for spent nuclear fuel.

Book AEC Research and Development Report

Download or read book AEC Research and Development Report written by Atomic Energy Commission and published by . This book was released on 1972 with total page 100 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Research and Development for Safeguards

Download or read book Research and Development for Safeguards written by Guy M. Inman and published by . This book was released on 1968 with total page 296 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Lead Slowing down Spectrometry Time Spectral Analysis for Spent Fuel Assay

Download or read book Lead Slowing down Spectrometry Time Spectral Analysis for Spent Fuel Assay written by and published by . This book was released on 2012 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Creating NDA Working Standards Through High fidelity Spent Fuel Modeling

Download or read book Creating NDA Working Standards Through High fidelity Spent Fuel Modeling written by and published by . This book was released on 2012 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: The Next Generation Safeguards Initiative (NGSI) is developing advanced non-destructive assay (NDA) techniques for spent nuclear fuel assemblies to advance the state-of-the-art in safeguards measurements. These measurements aim beyond the capabilities of existing methods to include the evaluation of plutonium and fissile material inventory, independent of operator declarations. Testing and evaluation of advanced NDA performance will require reference assemblies with well-characterized compositions to serve as working standards against which the NDA methods can be benchmarked and for uncertainty quantification. To support the development of standards for the NGSI spent fuel NDA project, high-fidelity modeling of irradiated fuel assemblies is being performed to characterize fuel compositions and radiation emission data. The assembly depletion simulations apply detailed operating history information and core simulation data as it is available to perform high fidelity axial and pin-by-pin fuel characterization for more than 1600 nuclides. The resulting pin-by-pin isotopic inventories are used to optimize the NDA measurements and provide information necessary to unfold and interpret the measurement data, e.g., passive gamma emitters, neutron emitters, neutron absorbers, and fissile content. A key requirement of this study is the analysis of uncertainties associated with the calculated compositions and signatures for the standard assemblies; uncertainties introduced by the calculation methods, nuclear data, and operating information. An integral part of this assessment involves the application of experimental data from destructive radiochemical assay to assess the uncertainty and bias in computed inventories, the impact of parameters such as assembly burnup gradients and burnable poisons, and the influence of neighboring assemblies on periphery rods. This paper will present the results of high fidelity assembly depletion modeling and uncertainty analysis from independent calculations performed using SCALE and MCNP. This work is supported by the Next Generation Safeguards Initiative, Office of Nuclear Safeguards and Security, National Nuclear Security Administration.

Book A Monte Carlo Based Spent Fuel Analysis Safeguards Strategy Assessment

Download or read book A Monte Carlo Based Spent Fuel Analysis Safeguards Strategy Assessment written by and published by . This book was released on 2009 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Safeguarding nuclear material involves the detection of diversions of significant quantities of nuclear materials, and the deterrence of such diversions by the risk of early detection. There are a variety of motivations for quantifying plutonium in spent fuel assemblies by means of nondestructive assay (NDA) including the following: strengthening the capabilities of the International Atomic Energy Agencies ability to safeguards nuclear facilities, shipper/receiver difference, input accountability at reprocessing facilities and burnup credit at repositories. Many NDA techniques exist for measuring signatures from spent fuel; however, no single NDA technique can, in isolation, quantify elemental plutonium and other actinides of interest in spent fuel. A study has been undertaken to determine the best integrated combination of cost effective techniques for quantifying plutonium mass in spent fuel for nuclear safeguards. A standardized assessment process was developed to compare the effective merits and faults of 12 different detection techniques in order to integrate a few techniques and to down-select among the techniques in preparation for experiments. The process involves generating a basis burnup/enrichment/cooling time dependent spent fuel assembly library, creating diversion scenarios, developing detector models and quantifying the capability of each NDA technique. Because hundreds of input and output files must be managed in the couplings of data transitions for the different facets of the assessment process, a graphical user interface (GUI) was development that automates the process. This GUI allows users to visually create diversion scenarios with varied replacement materials, and generate a MCNPX fixed source detector assessment input file. The end result of the assembly library assessment is to select a set of common source terms and diversion scenarios for quantifying the capability of each of the 12 NDA techniques. We present here the generalized assessment process, the techniques employed to automate the coupled facets of the assessment process, and the standard burnup/enrichment/cooling time dependent spent fuel assembly library. We also clearly define the diversion scenarios that will be analyzed during the standardized assessments. Though this study is currently limited to generic PWR assemblies, it is expected that the results of the assessment will yield an adequate spent fuel analysis strategy knowledge that will help the down-select process for other reactor types.

Book Methods and Techniques of NDA  nondestructive Assay

Download or read book Methods and Techniques of NDA nondestructive Assay written by and published by . This book was released on 1988 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Nondestructive assay (NDA) refers to techniques and instruments developed to measure nuclear materials in the many forms in which they occur throughout the fuel cycle. These techniques were first developed to support nuclear safeguards inspections and nuclear material accountability; they are also used extensively for process and quality control. Most accountability measurements are based on analytical chemistry and require that a sample be drawn and analyzed destructively. Destructive analysis can not be applied to many of the product materials found in the fuel cycle, such as fuel rods and assemblies, because of their high monetary value. Also, many waste and scrap materials can not be adequately sampled for destructive analysis because of their heterogenous nature. This situation led to the development of nondestructive analysis techniques. This paper presents an overview of the major NDA techniques and instrumentation in use today. The instrumentation described below is now used frequently by safeguards inspectors and facility operators alike. 19 refs., 18 figs., 4 tabs.

Book Lead Slowing down Spectrometry Time Spectral Analysis for Spent Fuel Assay

Download or read book Lead Slowing down Spectrometry Time Spectral Analysis for Spent Fuel Assay written by and published by . This book was released on 2011 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Developing a method for the accurate, direct, and independent assay of the fissile isotopes in bulk materials (such as used fuel) from next-generation domestic nuclear fuel cycles is a goal of the Office of Nuclear Energy, Fuel Cycle R & D, Material Protection and Control Technology (MPACT) Campaign. To meet this goal, MPACT supports a multi-institutional collaboration, of which PNNL is a part, to study the feasibility of Lead Slowing Down Spectroscopy (LSDS). This technique is an active nondestructive assay method that has the potential to provide independent, direct measurement of Pu and U isotopic masses in used fuel with an uncertainty considerably lower than the approximately 10% typical of today's confirmatory assay methods. This document is a progress report for FY2011 PNNL analysis and algorithm development. Progress made by PNNL in FY2011 continues to indicate the promise of LSDS analysis and algorithms applied to used fuel. PNNL developed an empirical model based on calibration of the LSDS to responses generated from well-characterized used fuel. The empirical model, which accounts for self-shielding effects using empirical basis vectors calculated from the singular value decomposition (SVD) of a matrix containing the true self-shielding functions of the used fuel assembly models. The potential for the direct and independent assay of the sum of the masses of 239Pu and 241Pu to within approximately 3% over a wide used fuel parameter space was demonstrated. Also, in FY2011, PNNL continued to develop an analytical model. Such efforts included the addition of six more non-fissile absorbers in the analytical shielding function and the non-uniformity of the neutron flux across the LSDS assay chamber. A hybrid analytical-empirical approach was developed to determine the mass of total Pu (sum of the masses of 239Pu, 240Pu, and 241Pu), which is an important quantity in safeguards. Results using this hybrid method were of approximately the same accuracy as the pure empirical approach. In addition, total Pu with much better accuracy with the hybrid approach than the pure analytical approach. In FY2012, PNNL will continue efforts to optimize its empirical model and minimize its reliance on calibration data. In addition, PNNL will continue to develop an analytical model, considering effects such as neutron-scattering in the fuel and cladding, as well as neutrons streaming through gaps between fuel pins in the fuel assembly.

Book Pre test Nondestructive Examination Data Summary Report on Turkey Point Spent Fuel Assemblies D01  D04 and D06 for the Climax   Spent Fuel Test

Download or read book Pre test Nondestructive Examination Data Summary Report on Turkey Point Spent Fuel Assemblies D01 D04 and D06 for the Climax Spent Fuel Test written by and published by . This book was released on 1981 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Safeguards Techniques and Equipment

Download or read book Safeguards Techniques and Equipment written by International Atomic Energy Agency and published by . This book was released on 2011 with total page 146 pages. Available in PDF, EPUB and Kindle. Book excerpt: The 1990s saw significant developments in the global non-proliferation landscape, resulting in a new period of safeguards development. The current publication, which is the second revision and update of IAEA/NVS/1, is intended to give a full and balanced description of the safeguards techniques and equipment used for nuclear material accountancy, containment and surveillance measures, environmental sampling, and data security. New features include a section on new and novel technologies. As new verification measures continue to be developed, the material in this book will be reviewed periodically and updated versions issued.

Book Nuclear Science Abstracts

Download or read book Nuclear Science Abstracts written by and published by . This book was released on 1976 with total page 612 pages. Available in PDF, EPUB and Kindle. Book excerpt:

Book Non destructive Assay of Spent Nuclear Fuel Using Passive Neutron Albedo Reactivity

Download or read book Non destructive Assay of Spent Nuclear Fuel Using Passive Neutron Albedo Reactivity written by and published by . This book was released on 2010 with total page pages. Available in PDF, EPUB and Kindle. Book excerpt: Passive Neutron Albedo Reactivity (PNAR) is one of fourteen techniques that has been researched and evaluated to form part of a comprehensive and integrated detection system for the non-destructive assay (NDA) of spent nuclear fuel. PNAR implemented with 3He tubes for neutron detection (PNAR-3He) is the measurement of time correlated neutrons from a spent fuel assembly with and without a Cadmium (Cd) layer surrounding the assembly. PNAR utilizes the self-interrogation of the fuel via reflection of neutrons born in the fuel assembly back in to the fuel assembly. The neutrons originate primarily from spontaneous fission events within the fuel itself (Curium-244) but are amplified by multiplication. The presence and removal of the Cd provides two measurement conditions with different neutron energy spectra and therefore different interrogating neutron characteristics. Cd has a high cross-section of absorption for slow neutrons and therefore greatly reduces the low energy (thermal) neutron fluence rate returning. The ratios of the Singles, Doubles and Triples count rates obtained in each case are known as the Cd ratios, which are related to fissile content. A potential safeguards application for which PNAR-3He is particularly suited is 'fingerprinting'. Fingerprinting could function as an alternative to plutonium (Pu) mass determination; providing confidence that material was not diverted during transport between sites. PNAR-3He has six primary NDA signatures: Singles, Doubles and Triples count rates measured with two energy spectra at both shipping and receiving sites. This is to uniquely identify the fuel assembly, and confirm no changes have taken place during transport. Changes may indicate all attempt to divert material for example. Here, the physics of the PNAR-3He concept will be explained, alongside a discussion on the development of a prototypical PNAR-3He instrument using simulation. The capabilities and performance of the conceptual instrument will be summarized, in the context of (a) quantifying Pu mass in spent fuel assemblies and (b) detecting pin diversion (through a discrepancy between declared and measured properties of the fuel assembly) when the instrument is deployed. These quantitative capabilities are complementary to the 'fingerprinting' capability which is part of ensuring continuity of knowledge and custody of spent nuclear fuel.